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@ARTICLE{Lon:18310,
author = {Léon, A. and Wuttke, J.},
title = {{H}ydrogen {R}elease from {S}odium {A}lanate {O}bserved by
{T}ime-resolved {N}eutron {B}ackscattering},
journal = {Journal of physics / Condensed matter},
volume = {23},
issn = {0953-8984},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {PreJuSER-18310},
pages = {254214},
year = {2011},
note = {Record converted from VDB: 12.11.2012},
abstract = {Innermolecular motion in Na(3)AlH(6) gives rise to a
Lorentzian spectrum with a wavenumber-independent width of
about 1 µeV at 180 °C, which is probably due to the
rotation of AlH(6) tetrahedra. There is no such quasielastic
line in NaAlH(4) or NaH. Based on this finding,
time-resolved measurements on the neutron backscattering
spectrometer SPHERES were used to monitor the decomposition
kinetics of sodium alanate, [Formula: see text] NaH. Both
reaction steps were found to be accelerated by
autocatalysis, most likely at the surfaces of Na(3)AlH(6)
and NaH crystallites.},
keywords = {J (WoSType)},
cin = {ICS-1 / JCNS (München) ; Jülich Centre for Neutron
Science JCNS (München) ; JCNS-FRM-II / JCNS-1 / JCNS-2},
ddc = {530},
cid = {I:(DE-Juel1)ICS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)JCNS-2-20110106},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung / Großgeräte für die Forschung
mit Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK415},
experiment = {EXP:(DE-MLZ)SPHERES-20140101},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:21654051},
UT = {WOS:000291433000017},
doi = {10.1088/0953-8984/23/25/254214},
url = {https://juser.fz-juelich.de/record/18310},
}