TY  - JOUR
AU  - Schubert, F.
AU  - Mokrousov, Y.
AU  - Ferriani, P.
AU  - Heinze, S.
TI  - Noncollinear magnetism in freestanding and supported monatomic Mn chains
JO  - Physical review / B
VL  - 83
IS  - 16
SN  - 1098-0121
CY  - College Park, Md.
PB  - APS
M1  - PreJuSER-18495
SP  - 165442
PY  - 2011
N1  - Financial support of the Stifterverband fur die Deutsche Wissenschaft is gratefully acknowledged. Y.M. thanks HGF-YIG Programme VH-NG-513 for funding and Julich Super-computing Center for computational time. We would like to thank Gustav Bihlmayer and especially Phivos Mavropoulos and Stefan Blugel for many illuminating discussions and suggestions.
AB  - Using first-principles calculations, we study the occurrence of noncollinear magnetic order in monatomic Mn chains. First, we focus on freestanding Mn chains and demonstrate that they exhibit a pronounced noncollinear ground state in a large range of interatomic distances between atoms in the chain. By artificially varying the atomic number of Mn we investigate how the magnetic ground state is influenced by alloying the Mn chains with Fe and Cr. With increasing number of 3d electrons we find a smooth transition in the magnetic phase space starting from an antiferromagnetic state for pure Cr chains through a regime of noncollinear ground states for Mn-rich chains to a ferromagnetic solution approaching the limit of pure Fe chains. Second, we investigate the magnetism in supported Mn chains on the (110) surfaces of Cu, Pd, and Ag. We show that even a weak chain-surface hybridization is sufficient to dramatically change the magnetic coupling in the chain. Nevertheless, while we observe that Mn chains are antiferromagnetic on Pd(110), a weak noncollinear magnetic order survives for Mn chains on Cu(110) and Ag(110) a few meV in energy below the antiferromagnetic solution. We explain the sensitive dependence of the exchange interaction in Mn chains on the interatomic distance, chemical composition, and their environment based on the competition between the ferromagnetic double exchange and the antiferromagnetic kinetic exchange mechanism. Finally, we perform simulations which predict that the noncollinear magnetic order of Mn chains on Cu(110) and Ag(110) could be experimentally verified by spin-polarized scanning tunneling microscopy.
KW  - J (WoSType)
LB  - PUB:(DE-HGF)16
UR  - <Go to ISI:>//WOS:000290115600007
DO  - DOI:10.1103/PhysRevB.83.165442
UR  - https://juser.fz-juelich.de/record/18495
ER  -