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000185521 0247_ $$2doi$$a10.5194/gmdd-7-7733-2014
000185521 0247_ $$2ISSN$$a1991-9611
000185521 0247_ $$2ISSN$$a1991-962X
000185521 0247_ $$2Handle$$a2128/8166
000185521 037__ $$aFZJ-2014-06948
000185521 082__ $$a910
000185521 1001_ $$0P:(DE-HGF)0$$aFlemming, J.$$b0$$eCorresponding Author
000185521 245__ $$aTropospheric chemistry in the integrated forecasting system of ECMWF
000185521 260__ $$aKatlenburg-Lindau$$bCopernicus$$c2014
000185521 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1420720149_16721
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000185521 520__ $$aA representation of atmospheric chemistry has been included in the Integrated Forecasting System (IFS) of the European Centre for Medium-range Weather Forecasts (ECMWF). The new chemistry modules complement the aerosol modules of the IFS for atmospheric composition, which is named C-IFS. C-IFS for chemistry supersedes a coupled system, in which the Chemical Transport Model (CTM) Model for OZone and Related chemical Tracers 3 was two-way coupled to the IFS (IFS-MOZART). This paper contains a description of the new on-line implementation, an evaluation with observations and a comparison of the performance of C-IFS with MOZART and with a re-analysis of atmospheric composition produced by IFS-MOZART within the Monitoring Atmospheric Composition and Climate (MACC) project. The chemical mechanism of C-IFS is an extended version of the Carbon Bond 2005 (CB05) chemical mechanism as implemented in the CTM Transport Model 5 (TM5). CB05 describes tropospheric chemistry with 54 species and 126 reactions. Wet deposition and lightning nitrogen monoxide (NO) emissions are modelled in C-IFS using the detailed input of the IFS physics package. A one-year simulation by C-IFS, MOZART and the MACC re-analysis is evaluated against ozonesondes, carbon monoxide (CO) aircraft profiles, European surface observations of ozone (O3), CO, sulphur dioxide (SO2) and nitrogen dioxide (NO2) as well as satellite retrievals of CO, tropospheric NO2 and formaldehyde. Anthropogenic emissions from the MACC/CityZen (MACCity) inventory and biomass burning emissions from the Global Fire Assimilation System (GFAS) data set were used in the simulations by both C-IFS and MOZART. C-IFS (CB05) showed an improved performance with respect to MOZART for CO, upper tropospheric O3, winter time SO2 and was of a similar accuracy for other evaluated species. C-IFS (CB05) is about ten times more computationally efficient than IFS-MOZART.
000185521 536__ $$0G:(DE-HGF)POF2-233$$a233 - Trace gas and aerosol processes in the troposphere (POF2-233)$$cPOF2-233$$fPOF II$$x0
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000185521 7001_ $$0P:(DE-HGF)0$$aHuijnen, V.$$b1
000185521 7001_ $$0P:(DE-HGF)0$$aArteta, J.$$b2
000185521 7001_ $$0P:(DE-HGF)0$$aBechtold, P.$$b3
000185521 7001_ $$0P:(DE-HGF)0$$aBeljaars, A.$$b4
000185521 7001_ $$0P:(DE-HGF)0$$aBlechschmidt, A.-M.$$b5
000185521 7001_ $$0P:(DE-HGF)0$$aJosse, B.$$b6
000185521 7001_ $$0P:(DE-HGF)0$$aDiamantakis, M.$$b7
000185521 7001_ $$0P:(DE-HGF)0$$aEngelen, R. J.$$b8
000185521 7001_ $$0P:(DE-HGF)0$$aGaudel, A.$$b9
000185521 7001_ $$0P:(DE-HGF)0$$aInness, A.$$b10
000185521 7001_ $$0P:(DE-HGF)0$$aJones, L.$$b11
000185521 7001_ $$0P:(DE-HGF)0$$aKatragkou, E.$$b12
000185521 7001_ $$0P:(DE-HGF)0$$aMarecal, V.$$b13
000185521 7001_ $$0P:(DE-HGF)0$$aPeuch, V.-H.$$b14
000185521 7001_ $$0P:(DE-HGF)0$$aRichter, A.$$b15
000185521 7001_ $$0P:(DE-Juel1)6952$$aSchultz, Martin$$b16$$ufzj
000185521 7001_ $$0P:(DE-Juel1)3709$$aStein, O.$$b17$$ufzj
000185521 7001_ $$0P:(DE-HGF)0$$aTsikerdekis, A.$$b18
000185521 773__ $$0PERI:(DE-600)2456729-2$$a10.5194/gmdd-7-7733-2014$$gVol. 7, no. 6, p. 7733 - 7803$$n6$$p7733 - 7803$$tGeoscientific model development discussions$$v7$$x1991-962X$$y2014
000185521 8564_ $$uwww.geosci-model-dev-discuss.net/7/7733/2014/
000185521 8564_ $$uhttps://juser.fz-juelich.de/record/185521/files/FZJ-2014-06948.pdf$$yOpenAccess
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000185521 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)3709$$aForschungszentrum Jülich GmbH$$b17$$kFZJ
000185521 9132_ $$0G:(DE-HGF)POF3-243$$1G:(DE-HGF)POF3-240$$2G:(DE-HGF)POF3-200$$aDE-HGF$$bMarine, Küsten- und Polare Systeme$$lAtmosphäre und Klima$$vTropospheric trace substances and their transformation processes$$x0
000185521 9131_ $$0G:(DE-HGF)POF2-233$$1G:(DE-HGF)POF2-230$$2G:(DE-HGF)POF2-200$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bErde und Umwelt$$lAtmosphäre und Klima$$vTrace gas and aerosol processes in the troposphere$$x0
000185521 9141_ $$y2014
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