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@PHDTHESIS{Nentwig:18561,
author = {Nentwig, Thomas},
title = {{E}xperimentelle {B}estimmung und numerische {S}imulation
von {V}iskositäten in {S}chlackesystemen unter
{V}ergasungsbedingungen},
volume = {129},
school = {RWTH Aachen},
type = {Dr. (Univ.)},
address = {Jülich},
publisher = {Forschungszentrum Jülich GmbH Zentralbibliothek, Verlag},
reportid = {PreJuSER-18561},
isbn = {978-3-89336-756-6},
series = {Schriften des Forschungszentrums Jülich : Energie $\&$
Umwelt / Energy $\&$ Environment},
pages = {XIII, 156, XV-LXXVI Seiten},
year = {2011},
note = {Record converted from JUWEL: 18.07.2013; RWTH Aachen,
Diss., 2011},
abstract = {Silica melts are reflected in many different industrial and
natural processes such as slags in steel production and
gasification of coal, glass in the glass making industry,
lava in the volcanology and in lots of other fields.
Rheological properties like the viscosity of this silica
melts are really important in all of these processes. A
general and good working viscosity model would help all
scientists and engineers, who have to simulate and optimise
these processes. First, it is important to have the
possibility to measure viscosities of slags. As part of this
PhD thesis a new high-temperature high-pressure rotational
viscosimeter is developed for measurements up to ≥1600 °C
and 20 bar. Particularly in relation to the coal
gasification process this two parameters are really
important, because coal gasification occurs under high
temperatures and high pressures. With this new viscosimeter
it is possible to measure slag viscosities under realistic
gasification conditions. To show that the new viscosimeter
works quite good viscosity measurements of four real slags
have been done. The influence of pressure and atmosphere on
viscosity have been examined. The measurements are also
compared with different viscosity models. The Arrhenius- and
Weymann-Equation have been determined and the correlation
between viscosity and basicity of the slag has been
evaluated. In the second part of the Phd thesis a new
viscosity model is developed. The model is based on the
structure inside the slag and consists in existing
thermodynamic models. After a detailed literature research
the model is developed for the
SiO$_{2}$-Al$_{2}$O$_{3}$-Na$_{2}$O-K$_{2}$O system. The
quality of this new model is estimated by comparing
calculated viscosity values with measurements found during
the literature research. The new model is also compared with
other existing models for viscosity calculation.},
cin = {IEK-2},
ddc = {500},
cid = {I:(DE-Juel1)IEK-2-20101013},
pnm = {Rationelle Energieumwandlung},
pid = {G:(DE-Juel1)FUEK402},
typ = {PUB:(DE-HGF)11 / PUB:(DE-HGF)3},
url = {https://juser.fz-juelich.de/record/18561},
}