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@INPROCEEDINGS{Lobe:186124,
author = {Lobe, Sandra and Stemme, Florian and Tsai, Chih-Long and
Finsterbusch, Martin and Dellen, Christian and Uhlenbruck,
Sven and Buchkremer, Hans Peter},
title = {{P}hysical vapor deposition of ${L}i_7{L}a_3{Z}r_2{O}_{12}$
for all-solid-state {L}i ion batteries},
reportid = {FZJ-2015-00212},
year = {2014},
abstract = {The liquid solvents used as electrolytes in conventional Li
ion batteries limit the operating temperature range and
cause safety problems due to insufficient electrochemical
stability. With purpose to avoid these disadvantages solid
electrolytes, like lithium conducting oxides, sulfides or
phosphates can be used. A promising oxide is the garnet-like
Li7La3Zr2O12 that shows one of the highest total Li ion
conductivities (about 10-4 S cm-1 at room temperature) in
this class of materials. It also enables a wide application
range due to its thermal stability and chemical resistance
against possible electrode materials, e.g. metallic
Lithium.In order to compensate the lower Li ion conductivity
compared to liquid electrolytes current work is focused on
thin electrolyte layers. Hence, main research aspect of the
presented work is the thin film processing of Li7La3Zr2O12
with physical vapor deposition methods, especially RF
magnetron sputtering. The growth conditions are optimized
with regard to synthesize stoichiometric, crack-free and
smooth thin films. Deposition is followed by thermal
treatment of the as-grown samples to improve the
crystallinity which should in turn improve the Li ion
conductivity. The composition, structure and the
electrochemical behavior of the resulting thin films are
analyzed in order to deposit all-solid-state thin film
batteries.},
month = {Jun},
date = {2014-06-10},
organization = {14th International Meeting on Lithium
Batteries, Como (Italy), 10 Jun 2014 -
14 Jun 2014},
cin = {IEK-1},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {123 - Fuel Cells (POF2-123) / HITEC - Helmholtz
Interdisciplinary Doctoral Training in Energy and Climate
Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF2-123 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)1},
url = {https://juser.fz-juelich.de/record/186124},
}