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000186334 0247_ $$2doi$$a10.1140/epje/i2014-14094-1
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000186334 1001_ $$0P:(DE-HGF)0$$aMaeda, Kousaku$$b0$$eCorresponding Author
000186334 245__ $$aHow does thermodiffusion of aqueous solutions depend on concentration and hydrophobicity?
000186334 260__ $$aBerlin$$bSpringer$$c2014
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000186334 520__ $$aThe thermal diffusion of aqueous solutions of mono-, di-ethylene glycols, poly(ethylene glycol), methanol, and glycerol is investigated systematically as a function of concentration using the Thermal Diffusion Forced Rayleigh Scattering (TDFRS). For all investigated binary mixtures, the Soret coefficient, S T , decays with increasing concentration of the non-aqueous component showing two regions. For aqueous solution of ethylene glycol, at a very low solute content the decay is steep, while it becomes less steep for higher solute concentration. All mixtures show a sign change of S T with concentration. The sign change concentration is discussed with respect to chemical structures of solute molecules and the partition coefficient, log p . It turns out that the number of hydroxyl groups plays an important role. For the investigated aqueous mixtures, we find empirical linear relations between the sign change concentration and the ratio of the number of hydroxyl groups to the number of carbon atoms as well as the partition coefficient, log p .
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000186334 7001_ $$0P:(DE-HGF)0$$aShinyashiki, Naoki$$b1
000186334 7001_ $$0P:(DE-HGF)0$$aYagihara, Shin$$b2
000186334 7001_ $$0P:(DE-Juel1)131034$$aWiegand, Simone$$b3$$ufzj
000186334 7001_ $$0P:(DE-HGF)0$$aKita, Rio$$b4
000186334 773__ $$0PERI:(DE-600)2004003-9$$a10.1140/epje/i2014-14094-1$$gVol. 37, no. 10, p. 94$$n10$$p94$$tThe @European physical journal / E$$v37$$x1292-895X$$y2014
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