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@ARTICLE{Maeda:186334,
      author       = {Maeda, Kousaku and Shinyashiki, Naoki and Yagihara, Shin
                      and Wiegand, Simone and Kita, Rio},
      title        = {{H}ow does thermodiffusion of aqueous solutions depend on
                      concentration and hydrophobicity?},
      journal      = {The European physical journal / E},
      volume       = {37},
      number       = {10},
      issn         = {1292-895X},
      address      = {Berlin},
      publisher    = {Springer},
      reportid     = {FZJ-2015-00410},
      pages        = {94},
      year         = {2014},
      abstract     = {The thermal diffusion of aqueous solutions of mono-,
                      di-ethylene glycols, poly(ethylene glycol), methanol, and
                      glycerol is investigated systematically as a function of
                      concentration using the Thermal Diffusion Forced Rayleigh
                      Scattering (TDFRS). For all investigated binary mixtures,
                      the Soret coefficient, S T , decays with increasing
                      concentration of the non-aqueous component showing two
                      regions. For aqueous solution of ethylene glycol, at a very
                      low solute content the decay is steep, while it becomes less
                      steep for higher solute concentration. All mixtures show a
                      sign change of S T with concentration. The sign change
                      concentration is discussed with respect to chemical
                      structures of solute molecules and the partition
                      coefficient, log p . It turns out that the number of
                      hydroxyl groups plays an important role. For the
                      investigated aqueous mixtures, we find empirical linear
                      relations between the sign change concentration and the
                      ratio of the number of hydroxyl groups to the number of
                      carbon atoms as well as the partition coefficient, log p .},
      cin          = {ICS-3},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ICS-3-20110106},
      pnm          = {451 - Soft Matter Composites (POF2-451)},
      pid          = {G:(DE-HGF)POF2-451},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000344339100001},
      doi          = {10.1140/epje/i2014-14094-1},
      url          = {https://juser.fz-juelich.de/record/186334},
}