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@ARTICLE{Crippa:186558,
author = {Crippa, M. and Canonaco, F. and Lanz, V. A. and Äijälä,
M. and Allan, J. D. and Carbone, S. and Capes, G. and
Ceburnis, D. and Dall'Osto, M. and Day, D. A. and DeCarlo,
P. F. and Ehn, M. and Eriksson, A. and Freney, E. and
Hildebrandt Ruiz, L. and Hillamo, R. and Jimenez, J. L. and
Junninen, H. and Kiendler-Scharr, A. and Kortelainen, A.-M.
and Kulmala, M. and Laaksonen, A. and Mensah, A. A. and
Mohr, C. and Nemitz, E. and O'Dowd, C. and Ovadnevaite, J.
and Pandis, S. N. and Petäjä, T. and Poulain, L. and
Saarikoski, S. and Sellegri, K. and Swietlicki, E. and
Tiitta, P. and Worsnop, D. R. and Baltensperger, U. and
Prévôt, A. S. H.},
title = {{O}rganic aerosol components derived from 25 {AMS} data
sets across {E}urope using a consistent {ME}-2 based source
apportionment approach},
journal = {Atmospheric chemistry and physics},
volume = {14},
number = {12},
issn = {1680-7324},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {FZJ-2015-00631},
pages = {6159 - 6176},
year = {2014},
abstract = {Organic aerosols (OA) represent one of the major
constituents of submicron particulate matter (PM1) and
comprise a huge variety of compounds emitted by different
sources. Three intensive measurement field campaigns to
investigate the aerosol chemical composition all over Europe
were carried out within the framework of the European
Integrated Project on Aerosol Cloud Climate and Air Quality
Interactions (EUCAARI) and the intensive campaigns of
European Monitoring and Evaluation Programme (EMEP) during
2008 (May–June and September–October) and 2009
(February–March). In this paper we focus on the
identification of the main organic aerosol sources and we
define a standardized methodology to perform source
apportionment using positive matrix factorization (PMF) with
the multilinear engine (ME-2) on Aerodyne aerosol mass
spectrometer (AMS) data. Our source apportionment procedure
is tested and applied on 25 data sets accounting for two
urban, several rural and remote and two high altitude sites;
therefore it is likely suitable for the treatment of
AMS-related ambient data sets. For most of the sites, four
organic components are retrieved, improving significantly
previous source apportionment results where only a
separation in primary and secondary OA sources was possible.
Generally, our solutions include two primary OA sources,
i.e. hydrocarbon-like OA (HOA) and biomass burning OA (BBOA)
and two secondary OA components, i.e. semi-volatile
oxygenated OA (SV-OOA) and low-volatility oxygenated OA
(LV-OOA). For specific sites cooking-related (COA) and
marine-related sources (MSA) are also separated. Finally,
our work provides a large overview of organic aerosol
sources in Europe and an interesting set of highly time
resolved data for modeling purposes.},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {233 - Trace gas and aerosol processes in the troposphere
(POF2-233)},
pid = {G:(DE-HGF)POF2-233},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000338438300019},
doi = {10.5194/acp-14-6159-2014},
url = {https://juser.fz-juelich.de/record/186558},
}