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@ARTICLE{Cao:187263,
author = {Cao, Chongde and Wildes, Andrew and Schmidt, Wolfgang and
Schmalzl, Karin and Hou, Binyang and Regnault, Louis-Pierre
and Zhang, Cong and Meuffels, Paul and Löser, Wolfgang and
Roth, Georg and Li, Haifeng},
title = {{D}istinct itinerant spin-density waves and local-moment
antiferromagnetism in an intermetallic {E}r{P}d2{S}i2 single
crystal},
journal = {Scientific reports},
volume = {5},
issn = {2045-2322},
address = {London},
publisher = {Nature Publishing Group},
reportid = {FZJ-2015-00936},
pages = {7968},
year = {2015},
abstract = {Identifying the nature of magnetism, itinerant or
localized, remains a major challenge in condensed-matter
science. Purely localized moments appear only in magnetic
insulators, whereas itinerant moments more or less co-exist
with localized moments in metallic compounds such as the
doped-cuprate or the iron-based superconductors, hampering a
thorough understanding of the role of magnetism in phenomena
like superconductivity or magnetoresistance. Here we
distinguish two antiferromagnetic modulations with
respective propagation wave vectors at Q± = (H ± 0.557(1),
0, L ± 0.150(1)) and QC = (H ± 0.564(1), 0, L), where (H,
L) are allowed Miller indices, in an ErPd2Si2 single crystal
by neutron scattering and establish their respective
temperature- and field-dependent phase diagrams. The
modulations can co-exist but also compete depending on
temperature or applied field strength. They couple
differently with the underlying lattice albeit with
associated moments in a common direction. The Q± modulation
may be attributed to localized 4f moments while the QC
correlates well with itinerant conduction bands, supported
by our transport studies. Hence, ErPd2Si2 represents a new
model compound that displays clearly-separated itinerant and
localized moments, substantiating early theoretical
predictions and providing a unique platform allowing the
study of itinerant electron behavior in a localized
antiferromagnetic matrix.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS-ILL / PGI-7},
ddc = {000},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-ILL-20110128 /
I:(DE-Juel1)PGI-7-20110106},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6213 - Materials
and Processes for Energy and Transport Technologies
(POF3-621) / 6G4 - Jülich Centre for Neutron Research
(JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6213 / G:(DE-HGF)POF3-6G4},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000348165800001},
doi = {10.1038/srep07968},
url = {https://juser.fz-juelich.de/record/187263},
}