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000187474 0247_ $$2doi$$a10.1103/PhysRevLett.113.268303
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000187474 1001_ $$0P:(DE-Juel1)129559$$aZhang, Jing$$b0$$eCorresponding Author$$ufzj
000187474 245__ $$aDirect Visualization of Conformation and Dense Packing of DNA-Based Soft Colloids
000187474 260__ $$aCollege Park, Md.$$bAPS$$c2014
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000187474 520__ $$aSoft colloids—such as polymer-coated particles, star polymers, block-copolymer micelles, microgels—constitute a broad class of materials where microscopic properties such as deformability and penetrability of the particle play a key role in tailoring their macroscopic properties which is of interest in many technological areas. The ability to access these microscopic properties is not yet demonstrated despite its great importance. Here we introduce novel DNA-coated colloids with star-shaped architecture that allows accessing the above local structural information by directly visualizing their intramolecular monomer density profile and arm’s free-end locations with confocal fluorescent microscopy. Compression experiments on a two-dimensional hexagonal lattice formed by these macromolecular assemblies reveal an exceptional resistance to mutual interpenetration of their charged corona at pressures approaching the MPa range. Furthermore, we find that this lattice, in a close packing configuration, is surprisingly tolerant to particle size variation. We anticipate that these stimuli-responsive materials could aid to get deeper insight in a wide range of problems in soft matter, including the study and design of biomimetic lubricated surfaces.
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000187474 7001_ $$0P:(DE-Juel1)130797$$aLettinga, M.P.$$b1$$ufzj
000187474 7001_ $$0P:(DE-Juel1)130616$$aDhont, Jan K.G.$$b2$$ufzj
000187474 7001_ $$0P:(DE-Juel1)130987$$aStiakakis, Emmanuel$$b3$$ufzj
000187474 773__ $$0PERI:(DE-600)1472655-5$$a10.1103/PhysRevLett.113.268303$$gVol. 113, no. 26, p. 268303$$n26$$p268303$$tPhysical review letters$$v113$$x0031-9007$$y2014
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000187474 9132_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
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