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@ARTICLE{Zinn:187533,
author = {Zinn, Thomas and Willner, Lutz and Lund, Reidar},
title = {{N}anoscopic {C}onfinement through {S}elf-{A}ssembly:
{C}rystallization within {M}icellar {C}ores {E}xhibits
{S}imple {G}ibbs-{T}homson {B}ehavior},
journal = {Physical review letters},
volume = {113},
number = {23},
issn = {1079-7114},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2015-01162},
pages = {238305},
year = {2014},
abstract = {It is well known that liquids confined to small nanoscopic
pores and droplets exhibit thermal behavior very different
from bulk samples. Less is known about liquids spontaneously
confined through self-assembly into micellar structures.
Here we demonstrate, using a very well-defined
n-alkyl-poly(ethylene oxide) polymer system with a tunable
structure, that n-alkane(s) forming 2–3 nm small micellar
cores are affected considerably by confinement in the form
of melting point depressions. Moreover, comparing the
reduction in melting points, ΔTm, determined through
volumetric and calorimetric methods with the micellar core
radius, Rc, obtained from small-angle x-ray scattering, we
find excellent agreement with the well-known Gibbs-Thomson
equation, ΔTm∼R−1c. This demonstrates that the reduced
size, i.e., the Laplace pressure, is the dominant parameter
governing the melting point depression in micellar systems.},
cin = {ICS-1 / Neutronenstreuung ; JCNS-1},
ddc = {550},
cid = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106},
pnm = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
(POF2-54G24)},
pid = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000346836400010},
doi = {10.1103/PhysRevLett.113.238305},
url = {https://juser.fz-juelich.de/record/187533},
}