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@ARTICLE{Mora:187677,
author = {Mora, Elsa and Bras, Ana and Pyckhout-Hintzen, Wim and
Diogo, Hermínio P. and Moura Ramos, Joaquim J.},
title = {{T}he segmental and chain relaxation modes in
high-cis-polyisoprene as studied by thermally stimulated
currents},
journal = {The journal of chemical physics},
volume = {142},
number = {4},
issn = {1089-7690},
address = {Melville, NY},
publisher = {American Institute of Physics},
reportid = {FZJ-2015-01303},
pages = {044903},
year = {2015},
abstract = {The technique of Thermally Stimulated Currents is used to
study the slow molecular mobility in a series of poly
(1,4-cis-isoprene) samples with different molecular weights,
Mw , and low polydispersity. The technique revealed a high
resolution power, particularly useful in the study of the
lower molecular weight samples where the chain and the
segmental relaxations strongly overlap. The dynamic
crossover that is reported for the normal mode by varying
the molecular weight is clearly revealed by the thermally
stimulated depolarization currents results through the
temperature location, TMn , of the normal mode peak, the
values of the relaxation time at TMn , τ(TMn ), and the
value of the fragility index of the normal mode, mn . The
kinetic features of the glass transition relaxation of
polyisoprene have also been determined.},
cin = {ICS-1 / Neutronenstreuung ; JCNS-1},
ddc = {540},
cid = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6215 - Soft Matter, Health and Life Sciences (POF3-621) /
551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6215 /
G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000349018100046},
doi = {10.1063/1.4906542},
url = {https://juser.fz-juelich.de/record/187677},
}