000187749 001__ 187749
000187749 005__ 20240619083507.0
000187749 0247_ $$2doi$$a10.1039/C4SM01935K
000187749 0247_ $$2ISSN$$a1744-683X
000187749 0247_ $$2ISSN$$a1744-6848
000187749 0247_ $$2Handle$$a2128/8387
000187749 0247_ $$2WOS$$aWOS:000345090400014
000187749 0247_ $$2altmetric$$aaltmetric:2827913
000187749 0247_ $$2pmid$$apmid:25351908
000187749 037__ $$aFZJ-2015-01340
000187749 041__ $$aEnglish
000187749 082__ $$a530
000187749 1001_ $$0P:(DE-HGF)0$$aVad, T.$$b0
000187749 245__ $$aSelf-assembly of biaxial discorectangular lead carbonate nanosheets into stacked ribbons studied by SAXS and HAADF-STEM tomographic tilt series
000187749 260__ $$aLondon$$bRoyal Soc. of Chemistry$$c2014
000187749 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1455697891_30101
000187749 3367_ $$2DataCite$$aOutput Types/Journal article
000187749 3367_ $$00$$2EndNote$$aJournal Article
000187749 3367_ $$2BibTeX$$aARTICLE
000187749 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000187749 3367_ $$2DRIVER$$aarticle
000187749 520__ $$aThe self-assembling behaviour of 2.6 nm thin PbCO3 nanoplatelets with discorectangular shape and uniform width and thickness occurring after their formation in nonionic water-in-oil microemulsions has been investigated using synchrotron small angle X-ray scattering (SAXS) and (scanning) transmission electron microscopy ((S)TEM). The presence of attractive depletion forces originating from the ubiquitous microemulsion droplets triggers a new type of superstructure at low particle concentration. Instead of the universally observed formation of face-to-face assembled lamellar mesostructures, the nanosheets self-organise into extended ribbon structures, whereby each on top lying sheet is displaced by a constant shift in the length and width directions leading to a so far unprecedented staggered zigzag-type stack assembly with restricted height. This type of stacking gives rise to a complex interference pattern in the isotropic small angle scattering of the stacked ribbon assemblies (SRAs) in reverse micellar solution. Different to the, for lamellar-structured nanosheets typical, diffraction peaks at multiples of the wave vector corresponding to one particular repeat distance, the scattering peaks measured in this study are asymmetric, displaying a shoulder on their low wave vector side. The asymmetric shape of the observed face-to-face correlation peaks indicates that the SRAs do not extend in one direction only. Their scattering behaviour is analysed by expanding the Kratky–Porod structure factor for stacking plates into three dimensions. High-angle annular dark-field (HAADF)-STEM tilt series have complementary been acquired to retrieve three-dimensional structural information on the SRAs in the dry state and to confirm the model used for the refinement of the SAXS data.
000187749 536__ $$0G:(DE-HGF)POF2-451$$a451 - Soft Matter Composites (POF2-451)$$cPOF2-451$$fPOF II$$x0
000187749 588__ $$aDataset connected to CrossRef, juser.fz-juelich.de
000187749 7001_ $$0P:(DE-HGF)0$$aHeidelmann, M.$$b1
000187749 7001_ $$0P:(DE-HGF)0$$aWeirich, T. E.$$b2
000187749 7001_ $$0P:(DE-Juel1)130932$$aSager, Wiebke$$b3$$eCorresponding Author
000187749 7001_ $$0P:(DE-Juel1)131058$$aZhang, Jing$$b4
000187749 773__ $$0PERI:(DE-600)2191476-X$$a10.1039/C4SM01935K$$gVol. 10, no. 47, p. 9511 - 9522$$n47$$p9511 - 9522$$tSoft matter$$v10$$x1744-6848$$y2014
000187749 8564_ $$uhttps://juser.fz-juelich.de/record/187749/files/FZJ-2015-01340.pdf$$yOpenAccess
000187749 909CO $$ooai:juser.fz-juelich.de:187749$$pdnbdelivery$$pVDB$$pdriver$$popen_access$$popenaire
000187749 915__ $$0LIC:(DE-HGF)CCBY3$$2HGFVOC$$aCreative Commons Attribution CC BY 3.0
000187749 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR
000187749 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000187749 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000187749 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000187749 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000187749 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000187749 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000187749 915__ $$0StatID:(DE-HGF)0400$$2StatID$$aAllianz-Lizenz / DFG
000187749 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz
000187749 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000187749 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000187749 915__ $$0StatID:(DE-HGF)9900$$2StatID$$aIF <  5
000187749 9141_ $$y2014
000187749 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)130932$$aForschungszentrum Jülich GmbH$$b3$$kFZJ
000187749 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)131058$$aForschungszentrum Jülich GmbH$$b4$$kFZJ
000187749 9132_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
000187749 9131_ $$0G:(DE-HGF)POF2-451$$1G:(DE-HGF)POF2-450$$2G:(DE-HGF)POF2-400$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bSchlüsseltechnologien$$lBioSoft$$vSoft Matter Composites$$x0
000187749 920__ $$lyes
000187749 9201_ $$0I:(DE-Juel1)ICS-3-20110106$$kICS-3$$lWeiche Materie$$x0
000187749 9201_ $$0I:(DE-Juel1)PGI-5-20110106$$kPGI-5$$lMikrostrukturforschung$$x1
000187749 9801_ $$aFullTexts
000187749 980__ $$ajournal
000187749 980__ $$aVDB
000187749 980__ $$aI:(DE-Juel1)ICS-3-20110106
000187749 980__ $$aI:(DE-Juel1)PGI-5-20110106
000187749 980__ $$aUNRESTRICTED
000187749 981__ $$aI:(DE-Juel1)ER-C-1-20170209
000187749 981__ $$aI:(DE-Juel1)PGI-5-20110106