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@ARTICLE{Du:188155,
author = {Du, Hongchu and Jia, Chun-Lin and Houben, Lothar and
Metlenko, Veronika and De Souza, Roger A. and Waser, R. and
Mayer, Joachim},
title = {{A}tomic structure and chemistry of dislocation cores at
low-angle tilt grain boundary in {S}r{T}i{O}3 bicrystals},
journal = {Acta materialia},
volume = {89},
issn = {1359-6454},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-01616},
pages = {344 - 351},
year = {2015},
abstract = {Dislocations in perovskite oxides have been found to have
important impacts on their electronic and ionic
transportation properties, which are believed to be related
to the structure and chemistry of dislocation cores. For
dislocation cores at a 6° low-angle [0 0 1] tilt grain
boundary in SrTiO3, an embedded TiOx rocksalt-like structure
has been suggested, consistent with a deficiency of Sr.
However, direct evidence supporting these suggestions has
not been obtained up to now. In this work, we reveal the
atomic structure and chemistry of edge dislocation cores at
a low-angle [0 0 1] symmetric tilt-boundary in SrTiO3
bicrystals by imaging techniques of high-angle annular
dark-field scanning transmission electron microscopy
(HAADF-STEM) and electron energy loss spectroscopy (EELS)
with an FEI Titan cube3 60–300 (PICO) microscope operated
at 80 kV. The experimental results demonstrate direct
evidence for a local coordination of edge-sharing TiO6
octahedra at the dislocation cores, which can be understood
as the result of strain. The local coordination of
edge-sharing TiO6 octahedra is associated with the
face-centered cubic (FCC) NaCl-type TiO phase. The present
study therefore provides a solid structural and chemical
basis for understanding the properties of dislocations.},
cin = {PGI-5 / PGI-7 / JARA-FIT},
ddc = {670},
cid = {I:(DE-Juel1)PGI-5-20110106 / I:(DE-Juel1)PGI-7-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000353249100033},
doi = {10.1016/j.actamat.2015.02.016},
url = {https://juser.fz-juelich.de/record/188155},
}