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@ARTICLE{Bram:188239,
      author       = {Bram, Martin and Brands, K. and Demeusy, L. and Zhao, Li
                      and Meulenberg, Wilhelm Albert and Pauls, J. and
                      Göttlicher, K. V. and Peinemann, S.},
      title        = {{T}esting of {N}ano-{S}tructured {G}as {S}eperation
                      {M}embranes in the {F}uel {G}as of a {P}ost-{C}ombustion
                      {P}ower {P}lant},
      journal      = {International journal of greenhouse gas control},
      volume       = {5},
      issn         = {1750-5836},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2015-01681},
      pages        = {37-48},
      year         = {2011},
      note         = {This project "Nano-structured ceramic and metal-supported
                      membranes for gas separation - METPORE" is founded by the
                      Bundeswirtschaftsministerium fur Wirtschaft und Technologie
                      (BMWi), Forderkennzeichen 0327746A. Funding is hereby
                      gratefully acknowledged. The authors would also like to
                      thank H.P. Hesse, K. Hassmann, North Rhine-Westphalia, EnBW,
                      E.ON and RWE for financial support and J. da Costa, D.
                      Uhlmann, University of Queensland, Brisbane, Australia, K.
                      Kroger, DVGW-Forschungstelle, University Karlsruhe, as well
                      as T. Van Gestel, F. Hauler, Ch. Somsen, W. Krumpen, D.
                      Sebold and W. Fischer, Forschungszentrum Julich, for their
                      help in preparation and characterisation of the membranes.},
      abstract     = {Nanostructured gas separation membranes are promising
                      candidates for the separation of CO2 from the flue gas of
                      fossil power plants. Well-defined atomic structures in the
                      range of a few Angstrom are required to separate CO2 from N2
                      in existing post-combustion power plants, and H2 from CO2 in
                      prospective integrated gasification combined cycle (IGCC)
                      power plants. Today, CO2/N2 and H2/CO2 gas separation with
                      membranes has been demonstrated mainly on a laboratory
                      scale, while less is known about membrane performance and
                      stability under real conditions. To extend the state of
                      knowledge, a test bed was put into operation in the flue gas
                      stream of a hard-coal-fired power plant (EnBW
                      Rheinhafendampfkraftwerk, Karlsruhe), which enabled the
                      long-term functional test of ceramic as well as polymer gas
                      separation membranes for up to 1100 h. For the first time, a
                      CO2 enrichment from 12 $vol.\%$ in the flue gas to 57
                      $vol.\%$ in the permeate of a polymer membrane was
                      demonstrated. Due to operating this membrane in direct
                      contact with flue gas, the flow rate was reduced from 0.86
                      to 0.07 m3/m2 h bar within the first 400 h. This reduction
                      was mainly caused by the deposition of ash particles and
                      gypsum suggesting the need of developing effective membrane
                      protection strategies. In addition, ceramic supported
                      Ti0.5Zr0.5O2 and metal supported Co–SiO2 membranes were
                      tested under the same conditions. Even if demonstration of
                      CO2 gas separation with ceramic membranes requires further
                      modifications of the membrane materials, the long-term
                      exposure in the power plant led to notable results regarding
                      adherence of functional layers and chemical stability.},
      cin          = {IEK-3 / IEK-1},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IEK-3-20101013 / I:(DE-Juel1)IEK-1-20101013},
      pnm          = {122 - Power Plants (POF2-122) / Rationelle
                      Energieumwandlung (FUEK402)},
      pid          = {G:(DE-HGF)POF2-122 / G:(DE-Juel1)FUEK402},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000287066700005},
      doi          = {WOS:000287066700005},
      url          = {https://juser.fz-juelich.de/record/188239},
}