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000188360 0247_ $$2doi$$a10.1016/j.ssi.2013.10.014
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000188360 1001_ $$0P:(DE-HGF)0$$aNozaki, Hiroshi$$b0$$eCorresponding Author
000188360 245__ $$aLi diffusive behavior of garnet-type oxides studied by muon-spin relaxation and QENS
000188360 260__ $$aAmsterdam [u.a.]$$bElsevier Science$$c2014
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000188360 520__ $$aA diffusive behavior of Li+ ion in a garnet-type oxide, Li5 + xLa3ZrxNb2 − x012 with x = 0–2, has been investigated by both a positive muon-spin relaxation (μ+SR) and quasi-elastic neutron scattering (QENS) technique using powder samples. The μ+SR results revealed that Li+ ions start to diffuse above ~ 150 K for the whole samples measured. The activation energy of Li diffusion (Ea) estimated from the μ+SR data was in good agreement with Ea obtained by the QENS measurements. However, both Eas were about a half of Ea of ionic conductivity of Li+ (σLi), which was evaluated by AC-impedance measurements on sintered pellets. This indicated the serious effect of grain boundary and/or surface on Ea. Furthermore, since the diffusion coefficient of Li+ estimated by μ+SR is roughly independent of x, the number of mobile Li+ in the garnet lattice was found to be the predominant parameter to determine σLi.
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000188360 7001_ $$0P:(DE-HGF)0$$aHarada, Masashi$$b1
000188360 7001_ $$0P:(DE-HGF)0$$aOhta, Shingo$$b2
000188360 7001_ $$0P:(DE-HGF)0$$aWatanabe, Isao$$b3
000188360 7001_ $$0P:(DE-HGF)0$$aMiyake, Yasuhiro$$b4
000188360 7001_ $$0P:(DE-HGF)0$$aIkedo, Yutaka$$b5
000188360 7001_ $$0P:(DE-Juel1)143752$$aJalarvo, Niina$$b6$$ufzj
000188360 7001_ $$0P:(DE-HGF)0$$aMamontov, Eugene$$b7
000188360 7001_ $$0P:(DE-HGF)0$$aSugiyama, Jun$$b8
000188360 773__ $$0PERI:(DE-600)1500750-9$$a10.1016/j.ssi.2013.10.014$$gVol. 262, p. 585 - 588$$p585 - 588$$tSolid state ionics$$v262$$x0167-2738$$y2014
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