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000188655 041__ $$aEnglish
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000188655 1001_ $$0P:(DE-Juel1)157720$$aLisicki, Maciej$$b0$$eCorresponding Author
000188655 245__ $$aTranslational and rotational near-wall diffusion of spherical colloids studied by evanescent wave scattering
000188655 260__ $$aLondon$$bRoyal Soc. of Chemistry$$c2014
000188655 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1426858592_11768
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000188655 520__ $$aIn this article we extend recent experimental developments [Rogers et al., Phys. Rev. Lett., 2012, 109, 098305] by providing a suitable theoretical framework for the derivation of exact expressions for the first cumulant (initial decay rate) of the correlation function measured in Evanescent Wave Dynamic Light Scattering (EWDLS) experiments. We focus on a dilute suspension of optically anisotropic spherical Brownian particles diffusing near a planar hard wall. In such a system, translational and rotational diffusion are hindered by hydrodynamic interactions with the boundary which reflects the flow incident upon it, affecting the motion of colloids. The validity of the approximation by the first cumulant for moderate times is assessed by juxtaposition to Brownian dynamics simulations, and compared with experimental results. The presented method for the analysis of experimental data allows the determination of penetration-depth-averaged rotational diffusion coefficients of spherical colloids at low density.
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000188655 7001_ $$0P:(DE-HGF)0$$aCichocki, Bogdan$$b1
000188655 7001_ $$0P:(DE-HGF)0$$aRogers, Simon A.$$b2
000188655 7001_ $$0P:(DE-Juel1)130616$$aDhont, Jan K.G.$$b3$$ufzj
000188655 7001_ $$0P:(DE-Juel1)130789$$aLang, Peter R.$$b4$$ufzj
000188655 773__ $$0PERI:(DE-600)2191476-X$$a10.1039/c4sm00148f$$gVol. 10, no. 24, p. 4312 -$$n24$$p4312$$tSoft matter$$v10$$x1744-6848$$y2014
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000188655 9132_ $$0G:(DE-HGF)POF3-551$$1G:(DE-HGF)POF3-550$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lBioSoft – Fundamentals for future Technologies in the fields of Soft Matter and Life Sciences$$vFunctional Macromolecules and Complexes$$x0
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