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000189120 1001_ $$0P:(DE-HGF)0$$aWalsh, Zarah$$b0$$eCorresponding Author
000189120 245__ $$aMultifunctional supramolecular polymer networks as next-generation consolidants for archaeological wood conservation
000189120 260__ $$aWashington, DC$$bNational Acad. of Sciences$$c2014
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000189120 520__ $$aThe preservation of our cultural heritage is of great importance to future generations. Despite this, significant problems have arisen with the conservation of waterlogged wooden artifacts. Three major issues facing conservators are structural instability on drying, biological degradation, and chemical degradation on account of Fe3+-catalyzed production of sulfuric and oxalic acid in the waterlogged timbers. Currently, no conservation treatment exists that effectively addresses all three issues simultaneously. A new conservation treatment is reported here based on a supramolecular polymer network constructed from natural polymers with dynamic cross-linking formed by a combination of both host-guest complexation and a strong siderophore pendant from a polymer backbone. Consequently, the proposed consolidant has the ability to chelate and trap iron while enhancing structural stability. The incorporation of antibacterial moieties through a dynamic covalent linkage into the network provides the material with improved biological resistance. Exploiting an environmentally compatible natural material with completely reversible chemistries is a safer, greener alternative to current strategies and may extend the lifetime of many culturally relevant waterlogged artifacts around the world. 
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000189120 65017 $$0V:(DE-MLZ)GC-170-2016$$2V:(DE-HGF)$$aEarth, Environment and Cultural Heritage$$x1
000189120 65017 $$0V:(DE-MLZ)GC-170$$2V:(DE-HGF)$$aEarth, Environment and Cultural Heritage $$x0
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000189120 7001_ $$0P:(DE-HGF)0$$aJaneček, Emma-Rose$$b1
000189120 7001_ $$0P:(DE-HGF)0$$aHodgkinson, James T.$$b2
000189120 7001_ $$0P:(DE-HGF)0$$aSedlmair, Julia$$b3
000189120 7001_ $$0P:(DE-Juel1)158075$$aKoutsioumpas, Alexandros$$b4
000189120 7001_ $$0P:(DE-HGF)0$$aSpring, David R.$$b5
000189120 7001_ $$0P:(DE-HGF)0$$aWelch, Martin$$b6
000189120 7001_ $$0P:(DE-HGF)0$$aHirschmugl, Carol J.$$b7
000189120 7001_ $$0P:(DE-HGF)0$$aToprakcioglu, Chris$$b8
000189120 7001_ $$0P:(DE-HGF)0$$aNitschke, Jonathan R.$$b9
000189120 7001_ $$0P:(DE-HGF)0$$aJones, Mark$$b10
000189120 7001_ $$0P:(DE-HGF)0$$aScherman, Oren A.$$b11
000189120 773__ $$0PERI:(DE-600)1461794-8$$a10.1073/pnas.1406037111$$gVol. 111, no. 50, p. 17743 - 17748$$n50$$p17743 - 17748$$tProceedings of the National Academy of Sciences of the United States of America$$v111$$x1091-6490$$y2014
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