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@ARTICLE{Flemming:189215,
author = {Flemming, J. and Huijnen, V. and Arteta, J. and Bechtold,
P. and Beljaars, A. and Blechschmidt, A.-M. and Diamantakis,
M. and Engelen, R. J. and Gaudel, A. and Inness, A. and
Jones, L. and Josse, B. and Katragkou, E. and Marecal, V.
and Peuch, V.-H. and Richter, A. and Schultz, Martin and
Stein, O. and Tsikerdekis, A.},
title = {{T}ropospheric chemistry in the {I}ntegrated {F}orecasting
{S}ystem of {ECMWF}},
journal = {Geoscientific model development},
volume = {8},
number = {4},
issn = {1991-9603},
address = {Katlenburg-Lindau},
publisher = {Copernicus},
reportid = {FZJ-2015-02406},
pages = {975 - 1003},
year = {2015},
abstract = {A representation of atmospheric chemistry has been included
in the Integrated Forecasting System (IFS) of the European
Centre for Medium-Range Weather Forecasts (ECMWF). The new
chemistry modules complement the aerosol modules of the IFS
for atmospheric composition, which is named C-IFS. C-IFS for
chemistry supersedes a coupled system in which chemical
transport model (CTM) Model for OZone and Related chemical
Tracers 3 was two-way coupled to the IFS (IFS-MOZART). This
paper contains a description of the new on-line
implementation, an evaluation with observations and a
comparison of the performance of C-IFS with MOZART and with
a re-analysis of atmospheric composition produced by
IFS-MOZART within the Monitoring Atmospheric Composition and
Climate (MACC) project. The chemical mechanism of C-IFS is
an extended version of the Carbon Bond 2005 (CB05) chemical
mechanism as implemented in CTM Transport Model 5 (TM5).
CB05 describes tropospheric chemistry with 54 species and
126 reactions. Wet deposition and lightning nitrogen
monoxide (NO) emissions are modelled in C-IFS using the
detailed input of the IFS physics package. A 1 year
simulation by C-IFS, MOZART and the MACC re-analysis is
evaluated against ozonesondes, carbon monoxide (CO) aircraft
profiles, European surface observations of ozone (O3), CO,
sulfur dioxide (SO2) and nitrogen dioxide (NO2) as well as
satellite retrievals of CO, tropospheric NO2 and
formaldehyde. Anthropogenic emissions from the MACC/CityZen
(MACCity) inventory and biomass burning emissions from the
Global Fire Assimilation System (GFAS) data set were used in
the simulations by both C-IFS and MOZART. C-IFS (CB05)
showed an improved performance with respect to MOZART for
CO, upper tropospheric O3, and wintertime SO2, and was of a
similar accuracy for other evaluated species. C-IFS (CB05)
is about 10 times more computationally efficient than
IFS-MOZART},
cin = {IEK-8 / JSC},
ddc = {910},
cid = {I:(DE-Juel1)IEK-8-20101013 / I:(DE-Juel1)JSC-20090406},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243) / 511 - Computational
Science and Mathematical Methods (POF3-511)},
pid = {G:(DE-HGF)POF3-243 / G:(DE-HGF)POF3-511},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000353841800003},
doi = {10.5194/gmd-8-975-2015},
url = {https://juser.fz-juelich.de/record/189215},
}