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@ARTICLE{PStoffel:189317,
author = {P Stoffel, Ralf and L Deringer, Volker and Dronskowski,
Richard and Simon, Ronnie and Hermann, Raphael},
title = {{A} density-functional study on the electronic and
vibrational properties of layered antimony telluride},
journal = {Journal of physics / Condensed matter},
volume = {27},
number = {8},
issn = {1361-648X},
address = {Bristol},
publisher = {IOP Publ.},
reportid = {FZJ-2015-02495},
pages = {085402},
year = {2015},
abstract = {We present a comprehensive survey of electronic and
lattice-dynamical properties of crystalline antimony
telluride (Sb2Te3). In a first step, the electronic
structure and chemical bonding have been investigated,
followed by calculations of the atomic force constants,
phonon dispersion relationships and densities of states.
Then, (macroscopic) physical properties of Sb2Te3 have been
computed, namely, the atomic thermal displacement
parameters, the Grüneisen parameter γ, the volume
expansion of the lattice, and finally the bulk modulus B. We
compare theoretical results from three popular and economic
density-functional theory (DFT) approaches: the local
density approximation (LDA), the generalized gradient
approximation (GGA), and a posteriori dispersion corrections
to the latter. Despite its simplicity, the LDA shows
excellent performance for all properties
investigated—including the Grüneisen parameter, which
only the LDA is able to recover with confidence. In the
absence of computationally more demanding hybrid DFT
methods, the LDA seems to be a good choice for further
lattice dynamical studies of Sb2Te3 and related layered
telluride materials.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JARA-HPC},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6213 - Materials
and Processes for Energy and Transport Technologies
(POF3-621) / 6G4 - Jülich Centre for Neutron Research
(JCNS) (POF3-623) / Chemical stability, oxidation, and
failure mechanisms of nanoscale phase-change memory
materials $(jara0033_20141101)$},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6213 / G:(DE-HGF)POF3-6G4 /
$G:(DE-Juel1)jara0033_20141101$},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000349605300010},
pubmed = {25662735},
doi = {10.1088/0953-8984/27/8/085402},
url = {https://juser.fz-juelich.de/record/189317},
}