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@ARTICLE{Tavabi:189387,
author = {Tavabi, Amir Hossein and Arai, S. and Muto, S. and Tanji,
T. and Dunin-Borkowski, Rafal},
title = {{I}n situ transmission electron microscopy of ionic
conductivity and reaction mechanism in ultrathin solid oxide
fuel cells},
journal = {Microscopy and microanalysis},
volume = {20},
number = {6},
issn = {1435-8115},
address = {New York, NY},
publisher = {Cambridge University Press},
reportid = {FZJ-2015-02562},
pages = {1817 - 1825},
year = {2014},
abstract = {Solid oxide fuel cells (SOFCs) are promising candidates for
use in alternative energy technologies. A full understanding
of the reaction mechanisms in these dynamic material systems
is required to optimize device performance and overcome
present limitations. Here, we show that in situ transmission
electron microscopy (TEM) can be used to study redox
reactions and ionic conductivity in SOFCs in a gas
environment at elevated temperature. We examine model
ultrathin half and complete cells in two environmental TEMs
using off-axis electron holography and electron energy-loss
spectroscopy. Our results from the model cells provide
insight into the essential phenomena that are important for
the operation of commercial devices. Changes in the
activities of dopant cations in the solid electrolyte are
detected during oxygen anion conduction, demonstrating the
key role of dopants in electrolyte architecture in SOFCs.},
cin = {PGI-5},
ddc = {570},
cid = {I:(DE-Juel1)PGI-5-20110106},
pnm = {42G - Peter Grünberg-Centre (PG-C) (POF2-42G41)},
pid = {G:(DE-HGF)POF2-42G41},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000347233400020},
doi = {10.1017/S143192761401349X},
url = {https://juser.fz-juelich.de/record/189387},
}