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000018975 084__ $$2WoS$$aChemistry, Physical
000018975 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000018975 084__ $$2WoS$$aPhysics, Multidisciplinary
000018975 084__ $$2WoS$$aPolymer Science
000018975 1001_ $$0P:(DE-Juel1)VDB97694$$aZinn, T.$$b0$$uFZJ
000018975 245__ $$aEquilibrium exchange kinetics in n-alkyl-PEO polymeric micelles: single exponential relaxation and chain length dependence
000018975 260__ $$aCambridge$$bRoyal Society of Chemistry (RSC)$$c2012
000018975 300__ $$a623 - 626
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000018975 520__ $$aIn this communication we present first results on the chain exchange kinetics of n-alkyl-PEO polymeric micelles by time-resolved small angle neutron scattering. We found that the rate strongly depends on the alkyl-chain length and that the relaxation function almost perfectly follows the single exponential decay predicted by theory. The key achievement of this study is the experimental verification that core block polydispersity accounts for the almost logarithmic time decay in block copolymer micelles as recently suggested by Choi et al. The results thus directly show that unimer exchange is the main mechanism for molecular exchange in block copolymer micelles.
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000018975 7001_ $$0P:(DE-Juel1)VDB4260$$aWillner, L.$$b1$$uFZJ
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000018975 8567_ $$uhttp://dx.doi.org/10.1039/C1SM06809A
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