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@ARTICLE{Sohn:190044,
author = {Sohn, Y. J. and Sparta, K. M. and Meven, M. and Roth, G.
and Heger, G.},
title = {{S}uperprotonic conductivity of
({NH}$_{4}$)$_{3}${H}({SO}$_{4}$)$_{2}$ in the
high-temperature phase},
journal = {Solid state ionics},
volume = {252},
issn = {0167-2738},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-03003},
pages = {116 - 120},
year = {2013},
abstract = {Impedance measurements were performed on single crystals of
(NH4)3H(SO4)2 in the temperature range of 295–441 K.
Anisotropy of protonic conductivity was found in the
monoclinic room-temperature phase (space group C2/c) as well
as in the rhombohedral high-temperature phase (space group R
3 ¯ m ). Above the high-temperature phase transition at 413
K, conductivity in the hexagonal (001) plane yields a value
of ~ 10− 2 S cm− 1, which is typical for superionic
conductors. A verification of a sample quality after the
impedance measurements, using X-ray powder diffraction,
showed minor additional peaks of (NH4)2(SO4). This suggests
a beginning of thermal decomposition at high temperature.
The possible pathways of proton conduction were discussed
according to crystal structure analyses by single-crystal
neutron diffraction method.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / JCNS-2 / IEK-1},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)IEK-1-20101013},
pnm = {422 - Spin-based and quantum information (POF2-422) / 424 -
Exploratory materials and phenomena (POF2-424) / 542 -
Neutrons (POF2-542) / 544 - In-house Research with PNI
(POF2-544) / 54G - JCNS (POF2-54G24)},
pid = {G:(DE-HGF)POF2-422 / G:(DE-HGF)POF2-424 /
G:(DE-HGF)POF2-542 / G:(DE-HGF)POF2-544 /
G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000328239600018},
doi = {10.1016/j.ssi.2013.06.011},
url = {https://juser.fz-juelich.de/record/190044},
}