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@ARTICLE{Gatta:190053,
author = {Gatta, G. Diego and Danisi, Rosa M. and Adamo, Ilaria and
Meven, Martin and Diella, Valeria},
title = {{A} single-crystal neutron and {X}-ray diffraction study of
elbaite},
journal = {Physics and chemistry of minerals},
volume = {39},
number = {7},
issn = {1432-2021},
address = {Berlin},
publisher = {Springer},
reportid = {FZJ-2015-03012},
pages = {577 - 588},
year = {2012},
abstract = {The crystal chemistry and crystal structure of gem-quality
elbaite from the Pederneira mine, São José da Safira,
Minas Gerais, Brazil, were investigated by electron
microprobe analysis in wavelength dispersive mode,
un-polarized Fourier transform infrared spectroscopy,
single-crystal neutron and X-ray diffraction. The average
chemical formula of the sample resulted X
(Na0.73Ca0.06□0.21) Y (Al1.24Li1.02Fe0.41Mn0.18Mg0.07) Z
Al6T Si6O18B (BO3)3V (OH)3W (OH0.46F0.54) and the chemical
analysis showed an almost homogeneous distribution of the
principal elements over the crystal, with significant
amounts of Fe $(wt\%$ FeO ~ 3.1) and Mn $(wt\%$ MnO ~ 1.3)
which substitute YAl. The infrared spectrum over the
diagnostic range of fundamental hydroxyl stretching
vibrations is characterized by three strong absorption bands
at 3,591 (ν1), 3,562 (ν2), and 3,491 (ν3) cm−1,
respectively. The neutron structure refinement showed: (a)
the presence of boron at the B site only and (b) the absence
(at a significant level) of aluminum at the T site, which
appears to be fully occupied by silicon. Only one proton
site was successfully located. The H bond configuration is
described with O3 as “donor” and O5 as “acceptor.”
The O3–H bond distance corrected for “riding motion”
is 0.9834 Å, and H···O5 = 2.238(7) Å, O3···O5 =
3.152(4) Å and O3–H···O5 = 157.7(5)°. The reasons of
the positional disorder at the O1 and O2 sites, observed in
both neutron and X-ray refinements, are discussed.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / JCNS-2},
ddc = {550},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {54G - JCNS (POF2-54G24)},
pid = {G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000305476900006},
doi = {10.1007/s00269-012-0513-0},
url = {https://juser.fz-juelich.de/record/190053},
}