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000019028 0247_ $$2DOI$$a10.1021/jp2018007
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000019028 084__ $$2WoS$$aChemistry, Physical
000019028 084__ $$2WoS$$aNanoscience & Nanotechnology
000019028 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000019028 1001_ $$0P:(DE-HGF)0$$aKowalzik, P.$$b0
000019028 245__ $$aSingle Electron Tunneling through a Tailored Arylthio-coronene
000019028 260__ $$aWashington, DC$$bSoc.$$c2011
000019028 300__ $$a9204 - 9209
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000019028 440_0 $$016841$$aJournal of Physical Chemistry C$$v115$$x1932-7447$$y18
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000019028 520__ $$aThe possibility to control the charge transport properties in molecular scale devices strongly depends upon the nature of the molecule metal interfaces, causing an intense request to engineer at molecular level the interface properties. Here, we report on single electron tunneling effects observed in a STM-tip/sing,le molecule/substrate device at room temperature using a molecule with a three-dimensional aromatic system. The molecule consists of a coronene core per-substituted with arylthio groups which are tailored in such a way that the aromatic system is efficiently decoupled from the metal substrate, and thus a double-barrier tunnel junction is created by means of a built-in insulating spacer. Comparing ab initio calculations with the experimental observations allows us to identify the specific arrangement of the substituents in the most stable conformer of this molecule. The tailored molecular structure in combination with the identified adsorption geometry controls the electron transport behavior and results in single electron transport features.
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000019028 7001_ $$0P:(DE-Juel1)131022$$aWaser, R.$$b5$$uFZJ
000019028 7001_ $$0P:(DE-Juel1)130751$$aKarthäuser, S.$$b6$$uFZJ
000019028 773__ $$0PERI:(DE-600)2256522-X$$a10.1021/jp2018007$$gVol. 115, p. 9204 - 9209$$p9204 - 9209$$q115<9204 - 9209$$tThe @journal of physical chemistry <Washington, DC> / C$$v115$$x1932-7447$$y2011
000019028 8567_ $$uhttp://dx.doi.org/10.1021/jp2018007
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