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@ARTICLE{Sen:19093,
author = {Sen, D. and Savio Melo, J: and Bahadur, J. and Mazumder, S.
and Bhattacharya, S. and D'Souza, S.F. and Frielinghaus, H.
and Goerigk, G. and Loidl, R.},
title = {{A}rrest of morphological transformation during
evaporation-induced self-assembly of mixed colloids in
micrometric droplets by charge tuning},
journal = {Soft matter},
volume = {7},
issn = {1744-683X},
address = {Cambridge},
publisher = {Royal Society of Chemistry (RSC)},
reportid = {PreJuSER-19093},
pages = {5423 - 5429},
year = {2011},
note = {Authors thank Dr S. Ramanathan of MSD, BARC for his kind
help in zeta-potential measurements. DS would like to thank
Drs Antoine Thill and Olivier Spalla of LIONS, SCM, DRECAM,
CEA Saclay, France for many fruitful discussions on spray
drying during his visit at CEA Saclay, France. DS and JB
thankfully acknowledge financial support
(DST(5)/AKR/P087/10-11/673) received from Department of
Science and Technology, India through S. N. Bose National
Centre for Basic Science, Kolkata, India for neutron
scattering work at JCNS, Germany and ILL, France.},
abstract = {Self-assembled grains of mixed colloids have been
synthesized using evaporation induced self-assembly (EISA)
by spray drying. We demonstrate using electron microscopy
and small-angle neutron scattering experiments that buckling
driven sphere to deformed-doughnut like morphological
transformation in such a process can be arrested by proper
tuning of the surface charge on the colloidal components.
The buckling amplitude diminishes with a reduction in
stabilization force between the colloidal particles. It is
established that such arrest of morphological transformation
is related to an effective exposure of the surface of softer
component at gas-liquid interface. Scattering experiments
confirm relatively more compact structure of the non-buckled
grains compared to that of the buckled grains. A plausible
mechanism regarding the arrest of morphological
transformation by surface charge tuning is illustrated.},
keywords = {J (WoSType)},
cin = {ICS-1 / JCNS (München) ; Jülich Centre for Neutron
Science JCNS (München) ; JCNS-FRM-II / JCNS-1},
ddc = {530},
cid = {I:(DE-Juel1)ICS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung / Großgeräte für die Forschung
mit Photonen, Neutronen und Ionen (PNI)},
pid = {G:(DE-Juel1)FUEK505 / G:(DE-Juel1)FUEK415},
experiment = {EXP:(DE-MLZ)KWS1-20140101 / EXP:(DE-MLZ)KWS3-20140101},
shelfmark = {Chemistry, Physical / Materials Science, Multidisciplinary
/ Physics, Multidisciplinary / Polymer Science},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000290937300045},
doi = {10.1039/c1sm05100h},
url = {https://juser.fz-juelich.de/record/19093},
}