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000019278 084__ $$2WoS$$aChemistry, Multidisciplinary
000019278 084__ $$2WoS$$aChemistry, Physical
000019278 084__ $$2WoS$$aMaterials Science, Multidisciplinary
000019278 1001_ $$0P:(DE-HGF)0$$aBahadur, J.$$b0
000019278 245__ $$aOrigin of Buckling Phenomenon during Drying of Micrometer-Sized Colloidal Droplets
000019278 260__ $$aWashington, DC$$bACS Publ.$$c2011
000019278 300__ $$a8404 - 8414
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000019278 440_0 $$04081$$aLangmuir$$v27$$x0743-7463
000019278 500__ $$aThe authors thankfully acknowledge financial support [DST (5)/AKR/P087/10-11/673] received from Department of Science and Technology, India, through the S. N. Bose National Centre for Basic Science, Kolkata, India, for neutron scattering work at JCNS, Garching, Germany.
000019278 520__ $$aThe origin of the buckling of micrometer-sized colloidal droplets during evaporation-induced self-assembly (EISA) has been elucidated using electron microscopy and small-angle neutron scattering. Doughnut-like assembled grains with varying aspect ratios are formed during EISA at different physicochemical conditions. It has been revealed that this phenomenon is better explained by an existing hypothesis based on the formation of a viscoelastic shell of nanoparticles during drying than by other existing hypotheses based on the inertial instability of the initial droplets and hydrodynamic instability due to thermocapillary forces. This conclusion was further supported by the arrest of buckling through modification of the colloidal interaction in the initial dispersion.
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000019278 7001_ $$0P:(DE-HGF)0$$aSen, D.$$b1
000019278 7001_ $$0P:(DE-HGF)0$$aMazumder, S.$$b2
000019278 7001_ $$0P:(DE-HGF)0$$aBhattacharya, S.$$b3
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000019278 8567_ $$uhttp://dx.doi.org/10.1021/la200827n
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