Hauptseite > Publikationsdatenbank > Anisotropic Pair Correlations and Structure Factors of Confined Hard-Sphere Fluids: An Experimental and Theoretical Study > print

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|a 10.1103/PhysRevLett.108.037802
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100 1 _ |0 P:(DE-HGF)0
|a Nygard, K.
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245 _ _ |a Anisotropic Pair Correlations and Structure Factors of Confined Hard-Sphere Fluids: An Experimental and Theoretical Study
260 _ _ |a College Park, Md.
|b APS
|c 2012
300 _ _ |a 037802
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440 _ 0 |0 4925
|a Physical Review Letters
|v 108
|x 0031-9007
|y 3
500 _ _ |a The experiment was carried out at the cSAXS beam line of the Swiss Light Source, Paul Scherrer Institut, Villigen, Switzerland. We thank the beam line staff for assistance. One of us (R. K.) gratefully acknowledges support from the Swedish Research council. The calculations in this work were supported by the Swedish National Infrastructure for Computing (SNIC 001-09-152) via PDC.
520 _ _ |a We address the fundamental question: how are pair correlations and structure factors of hard-sphere fluids affected by confinement between hard planar walls at close distance? For this purpose, we combine x-ray scattering from colloid-filled nanofluidic channel arrays and first-principles inhomogeneous liquid-state theory within the anisotropic Percus-Yevick approximation. The experimental and theoretical data are in remarkable agreement at the pair-correlation level, providing the first quantitative experimental verification of the theoretically predicted confinement-induced anisotropy of the pair-correlation functions for the fluid. The description of confined fluids at this level provides, in the general case, important insights into the mechanisms of particle-particle interactions in dense fluids under confinement.
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856 7 _ |u http://dx.doi.org/10.1103/PhysRevLett.108.037802
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