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@ARTICLE{Kleusch:19786,
author = {Kleusch, C. and Hersch, N. and Hoffmann, B. and Merkel, R.
and Csiszar, A.},
title = {{F}luorescent lipids: functional parts of fusogenic
liposomes and tools for cell membrane labeling and
visualization},
journal = {Molecules},
volume = {17},
issn = {1420-3049},
address = {Basel},
publisher = {MDPI},
reportid = {PreJuSER-19786},
pages = {1055 - 1073},
year = {2012},
note = {We thank Gerhild van Echten-Deckert for helpful discussions
and Simon Ludwanowski, who produced many of the fusogenic
liposomes used in this study. Our work was fully funded by
the Helmholtz Association.},
abstract = {In this paper a rapid and highly efficient method for
controlled incorporation of fluorescent lipids into living
mammalian cells is introduced. Here, the fluorescent
molecules have two consecutive functions: First, they
trigger rapid membrane fusion between cellular plasma
membranes and the lipid bilayers of their carrier particles,
so called fusogenic liposomes, and second, after insertion
into cellular membranes these molecules enable fluorescence
imaging of cell membranes and membrane traffic processes. We
tested the fluorescent derivatives of the following
essential membrane lipids for membrane fusion: Ceramide,
sphingomyelin, phosphocholine,
phosphatidylinositol-bisphosphate, ganglioside, cholesterol,
and cholesteryl ester. Our results show that all probed
lipids could more efficiently be incorporated into the
plasma membrane of living cells than by using other methods.
Moreover, labeling occurred in a gentle manner under
classical cell culture conditions reducing cellular stress
responses. Staining procedures were monitored by
fluorescence microscopy and it was observed that
sphingolipids and cholesterol containing free hydroxyl
groups exhibit a decreased distribution velocity as well as
a longer persistence in the plasma membrane compared to
lipids without hydroxyl groups like phospholipids or other
artificial lipid analogs. After membrane staining, the
fluorescent molecules were sorted into membranes of cell
organelles according to their chemical properties and
biological functions without any influence of the delivery
system.},
keywords = {Animals / CHO Cells / Cell Membrane: chemistry / Cell
Survival: drug effects / Cricetinae / Fibroblasts: chemistry
/ Fluorescent Dyes: chemistry / Intracellular Membranes:
chemistry / Liposomes: chemistry / Membrane Fusion: drug
effects / Membrane Lipids: chemistry / Membrane Lipids:
pharmacology / Organelles: chemistry / Rats / Rats, Wistar /
Staining and Labeling: methods / Fluorescent Dyes (NLM
Chemicals) / Liposomes (NLM Chemicals) / Membrane Lipids
(NLM Chemicals) / J (WoSType)},
cin = {ICS-7},
ddc = {540},
cid = {I:(DE-Juel1)ICS-7-20110106},
pnm = {BioSoft: Makromolekulare Systeme und biologische
Informationsverarbeitung},
pid = {G:(DE-Juel1)FUEK505},
shelfmark = {Chemistry, Organic},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:22267193},
UT = {WOS:000299535700072},
doi = {10.3390/molecules17011055},
url = {https://juser.fz-juelich.de/record/19786},
}