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@ARTICLE{Reitz:19850,
author = {Reitz, P. and Spindler, C. and Mentel, T.F. and Poulain, L.
and Wex, H. and Mildenberger, K. and Niedermeier, D. and
Hartmann, S. and Clauss, T. and Stratmann, F. and Sullivan,
R.C. and DeMott, P.J. and Petters, M.D. and Sierau, B. and
Schneider, J.},
title = {{S}urface modification of mineral dust particles by
sulphuric acid processing: implications for ice nucleation
abilities},
journal = {Atmospheric chemistry and physics},
volume = {11},
issn = {1680-7316},
address = {Katlenburg-Lindau},
publisher = {EGU},
reportid = {PreJuSER-19850},
pages = {7839 - 7858},
year = {2011},
note = {This work was conducted within the Helmholtz virtual
institute on aerosol cloud interaction and supported by the
Integration of European Simulation Chambers for
Investigating Atmospheric Processes (EUROCHAMP) program as
well as by the US National Science Foundation (Grant
ATM-0611936). We thank all the participants of the FROST
campaigns for their support and valuable discussions.},
abstract = {The ability of coated mineral dust particles to act as ice
nuclei (IN) was investigated at LACIS (Leipzig Aerosol Cloud
Interaction Simulator) during the FROST1- and
FROST2-campaigns (Freezing of dust). Sulphuric acid was
condensed on the particles which afterwards were optionally
humidified, treated with ammonia vapour and/or heat. By
means of aerosol mass spectrometry we found evidence that
processing of mineral dust particles with sulphuric acid
leads to surface modifications of the particles. These
surface modifications are most likely responsible for the
observed reduction of the IN activation of the particles.
The observed particle mass spectra suggest that different
treatments lead to different chemical reactions on the
particle surface. Possible chemical reaction pathways and
products are suggested and the implications on the IN
efficiency of the treated dust particles are discussed.},
keywords = {J (WoSType)},
cin = {IEK-8},
ddc = {550},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {Atmosphäre und Klima},
pid = {G:(DE-Juel1)FUEK491},
shelfmark = {Meteorology $\&$ Atmospheric Sciences},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000293826500026},
doi = {10.5194/acp-11-7839-2011},
url = {https://juser.fz-juelich.de/record/19850},
}