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@ARTICLE{Ibach:201029,
      author       = {Ibach, Harald},
      title        = {{V}ibration spectroscopy of water on stepped gold surfaces},
      journal      = {Surface science},
      volume       = {604},
      number       = {3-4},
      issn         = {0039-6028},
      address      = {Amsterdam},
      publisher    = {Elsevier},
      reportid     = {FZJ-2015-03339},
      pages        = {377 - 385},
      year         = {2010},
      abstract     = {The vibration spectrum of H2O (ice) adsorbed at low
                      temperatures on Au(1 0 0), Au(1 11 1), and Au(1 1 5) is
                      studied using electron energy loss spectroscopy. On the Au(1
                      0 0) surface, the spectra show the presence of the typical
                      H-bonded network of water molecules for all coverages from
                      the submonolayer into the multilayer range. The absence of a
                      non-H-bonded OH-stretching mode is indicative for the
                      “H-down bilayer”. On stepped surfaces, on the other
                      hand, a considerable fraction of the H-atoms remains in the
                      non-H-bonded state; surprisingly even in the multilayer
                      range, and even after annealing. The fraction of
                      non-H-bonded hydrogen atoms scales with the step density.
                      Spectral features of water adsorbed at step-sites are
                      isolated after annealing a surface exposed to small doses of
                      H2O. The results are discussed in the context of recent
                      theoretical studies as well as in conceivable relation to
                      the experimentally found reduction of the
                      Helmholtz-capacitance on stepped Au(1 1 n) electrodes.},
      cin          = {PGI-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)PGI-3-20110106},
      pnm          = {422 - Spin-based and quantum information (POF2-422)},
      pid          = {G:(DE-HGF)POF2-422},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000274979000021},
      doi          = {10.1016/j.susc.2009.11.034},
      url          = {https://juser.fz-juelich.de/record/201029},
}