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@ARTICLE{Schwarz:201033,
author = {Schwarz, Daniel and van Gastel, R. and Zandvliet, HJW and
Poelsema, B.},
title = {{G}rowth {A}nomalies in {S}upramolecular {N}etworks: 4,4
'-{B}iphenyldicarboxylic {A}cid on {C}u(001)},
journal = {Physical review letters},
volume = {110},
number = {7},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2015-03343},
pages = {076101},
year = {2013},
abstract = {We have used low energy electron microscopy to demonstrate
how the interaction of 4,4′-biphenyldicarboxylic acid
(BDA) molecules with (steps on) the Cu(001) surface
determines the structure of supramolecular BDA networks on a
mesoscopic length scale. Our in situ real time observations
reveal that steps are permeable to individual molecules but
that the change in crystal registry between different layers
of the Cu substrate causes them to be completely impermeable
to condensed BDA domains. The resulting growth instabilities
determine the evolution of the domain shape and include a
novel Mullins-Sekerka-type growth instability that is
characterized by high growth rates along, instead of
perpendicular to, the Cu steps. This growth instability is
responsible for the majority of residual defects in the BDA
networks.},
cin = {PGI-3},
ddc = {550},
cid = {I:(DE-Juel1)PGI-3-20110106},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000314995400005},
doi = {10.1103/PhysRevLett.110.076101},
url = {https://juser.fz-juelich.de/record/201033},
}