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@ARTICLE{MeierKoll:201060,
      author       = {Meier-Koll, Andreas and Pipich, Vitaliy and Busch, Peter
                      and Papadakis, Christine M. and Müller-Buschbaum, Peter},
      title        = {{P}hase {S}eparation in {S}emidilute {A}queous {P}oly( {N}
                      -isopropylacrylamide) {S}olutions},
      journal      = {Langmuir},
      volume       = {28},
      number       = {23},
      issn         = {1520-5827},
      address      = {Washington, DC},
      publisher    = {ACS Publ.},
      reportid     = {FZJ-2015-03370},
      pages        = {8791 - 8798},
      year         = {2012},
      abstract     = {The phase separation mechanism in semidilute aqueous
                      poly(N-isopropylacrylamide) (PNIPAM) solutions is
                      investigated with small-angle neutron scattering (SANS). The
                      nature of the phase transition is probed in static SANS
                      measurements and with time-dependent SANS measurements after
                      a temperature jump. The observed critical exponents of the
                      phase transition describing the temperature dependence of
                      the Ornstein–Zernike amplitude and correlation length are
                      smaller than values from mean-field theory. Time-dependent
                      SANS measurements show that the specific surface decreases
                      with increasing time after a temperature jump above the
                      phase transition. Thus, the formation of additional hydrogen
                      bonds in the collapsed state is a kinetic effect: A certain
                      fraction of water remains as bound water in the system.
                      Moreover, H–D exchange reactions observed in PNIPAM have
                      to be taken into account.},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {670},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {54G - JCNS (POF2-54G24)},
      pid          = {G:(DE-HGF)POF2-54G24},
      experiment   = {EXP:(DE-MLZ)KWS2-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000305092700024},
      doi          = {10.1021/la3015332},
      url          = {https://juser.fz-juelich.de/record/201060},
}