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000201069 1001_ $$0P:(DE-HGF)0$$aPaul, N.$$b0$$eCorresponding Author
000201069 245__ $$aInterfacial smoothening of polymer multilayers with molecules: a new approach in growing supramolecular layer structures
000201069 260__ $$aLondon$$bRoyal Soc. of Chemistry$$c2013
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000201069 520__ $$aThe development of polymer-based structures is hindered due to the difficulties in realizing well-defined modulated structures without interpenetration of charged polymers. Two types of polyelectrolyte multilayer structures, with and without embedded layers of the biomolecule, glutamic acid, are compared using infrared spectroscopy and X-ray and neutron scattering techniques. Structure characterization of polyelectrolyte multilayers focuses usually on the arrangement along the surface normal. Using specular and off-specular neutron scattering we get insight into the in- and out-of-plane arrangement of the structure. A formation of well-defined, smooth layers is observed in the structure containing the biomolecule. This reduced roughness is associated with a drastic decrease in chain mobility responsible for interpenetration. In contrast, the multilayer without the biomolecule forms an island-like structure. Thus biomolecules can interrupt the propagation of island-like structures at such interfaces which can be effectively used in achieving well-defined supramolecular layer structures out of charged polymers.
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000201069 7001_ $$0P:(DE-HGF)0$$aPaul, A.$$b1
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000201069 7001_ $$0P:(DE-HGF)0$$aBöni, P.$$b4
000201069 7001_ $$0P:(DE-HGF)0$$aLux-Steiner, M. Ch.$$b5
000201069 773__ $$0PERI:(DE-600)2191476-X$$a10.1039/c3sm51792f$$gVol. 9, no. 42, p. 10117 -$$n42$$p10117-10128$$tSoft matter$$v9$$x1744-6848$$y2013
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