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@ARTICLE{Paul:201069,
      author       = {Paul, N. and Paul, A. and Mattauch, S. and
                      Müller-Buschbaum, P. and Böni, P. and Lux-Steiner, M. Ch.},
      title        = {{I}nterfacial smoothening of polymer multilayers with
                      molecules: a new approach in growing supramolecular layer
                      structures},
      journal      = {Soft matter},
      volume       = {9},
      number       = {42},
      issn         = {1744-6848},
      address      = {London},
      publisher    = {Royal Soc. of Chemistry},
      reportid     = {FZJ-2015-03379},
      pages        = {10117-10128},
      year         = {2013},
      abstract     = {The development of polymer-based structures is hindered due
                      to the difficulties in realizing well-defined modulated
                      structures without interpenetration of charged polymers. Two
                      types of polyelectrolyte multilayer structures, with and
                      without embedded layers of the biomolecule, glutamic acid,
                      are compared using infrared spectroscopy and X-ray and
                      neutron scattering techniques. Structure characterization of
                      polyelectrolyte multilayers focuses usually on the
                      arrangement along the surface normal. Using specular and
                      off-specular neutron scattering we get insight into the in-
                      and out-of-plane arrangement of the structure. A formation
                      of well-defined, smooth layers is observed in the structure
                      containing the biomolecule. This reduced roughness is
                      associated with a drastic decrease in chain mobility
                      responsible for interpenetration. In contrast, the
                      multilayer without the biomolecule forms an island-like
                      structure. Thus biomolecules can interrupt the propagation
                      of island-like structures at such interfaces which can be
                      effectively used in achieving well-defined supramolecular
                      layer structures out of charged polymers.},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {530},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {451 - Soft Matter Composites (POF2-451) / 54G - JCNS
                      (POF2-54G24)},
      pid          = {G:(DE-HGF)POF2-451 / G:(DE-HGF)POF2-54G24},
      experiment   = {EXP:(DE-MLZ)TREFF-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000325726100018},
      doi          = {10.1039/c3sm51792f},
      url          = {https://juser.fz-juelich.de/record/201069},
}