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@ARTICLE{Wojciechowski:201083,
author = {Wojciechowski, Kamil and Gutberlet, Thomas and Konovalov,
Oleg},
title = {{A}nion-specificity at water–air interface probed by
total reflection {X}-ray fluorescence ({TRXF})},
journal = {Colloids and surfaces / A},
volume = {413},
issn = {0927-7757},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2015-03393},
pages = {184 - 190},
year = {2012},
abstract = {Accumulation of bromide ions in the Stern part of the
electrical double layer (EDL) near a Gibbs monolayer of
cationic surfactant, cetyltrimethylammonium bromide (CTABr),
at the water–air interface was probed by the total
reflection X-ray fluorescence (TRXF). A combination of TRXF
with surface tension data allowed for the first time to
determine the adsorbed amounts of bromide ions in the Stern
and diffuse parts of EDL. TRXF and X-ray reflectivity (XR)
were employed to probe the competitive adsorption of other
anions present in the aqueous solution. The Gibbs monolayers
of CTABr were studied in the absence and presence of
different anions from the Hofmeister series (Br−, NO3−,
F−, Cl−, H2PO4−, ClO4−, and I−) with the aim to
compare their affinity to the interface positively charged
by adsorption of surface-active CTA+ cation. For studying
the effect of anions on adsorption of CTABr, the
concentration of the latter was kept constant (10−4 M),
and that of NaX (X− = Br−, NO3−, F−, Cl−,
H2PO4−, ClO4−, and I−) was varied between 10−2 M and
10−5 M. The results clearly show the competition between
anions for the positively charged aqueous–air interface,
with F− being the least “surface active” and ClO4−
and I− – the most “surface active” anions, in full
agreement with the Hofmeister series.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1 /
JCNS-2},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106 / I:(DE-Juel1)JCNS-2-20110106},
pnm = {54G - JCNS (POF2-54G24)},
pid = {G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000310184400030},
doi = {10.1016/j.colsurfa.2012.06.045},
url = {https://juser.fz-juelich.de/record/201083},
}