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@ARTICLE{Sawinski:201202,
author = {Sawinski, Peter Klaus and Meven, Martin and Englert, Ulli
and Dronskowski, Richard},
title = {{S}ingle-{C}rystal {N}eutron {D}iffraction {S}tudy on
{G}uanidine, {CN} $_{3}$ {H} $_{5}$},
journal = {Crystal growth $\&$ design},
volume = {13},
number = {4},
issn = {1528-7505},
address = {Washington, DC},
publisher = {ACS Publ.},
reportid = {FZJ-2015-03507},
pages = {1730 - 1735},
year = {2013},
abstract = {Pure guanidine crystallizes in the orthorhombic space group
Pbca (no. 61) and a = 8.5022(2) Å, b = 9.0863(2) Å, c =
15.6786(4) Å at 100 K, Z = 16, with two Y-shaped molecules
in the asymmetric unit. The compound features a
three-dimensional network of classical N–H···N hydrogen
bonds. Here, we present the results of a single-crystal
neutron diffraction study, performed at two different
temperatures (100 and 273 K). The data quality obtained at
the HEiDi instrument (FRM II, Munich) allowed to derive
accurate positional and anisotropic displacement parameters
(ADP) for all the atoms, including H. The experimental
hydrogen positions confirm a model derived from theory. On
the basis of the displacement parameters, a TLS analysis of
thermal motion proves that the guanidine molecules behave in
good approximation as rigid bodies and essentially undergo
libration. The unusual temperature behavior of one C–N
bond found in a preceding single-crystal X-ray study is an
artifact going back to this rigid-body movement. The
existence of various hydrogen bonds also manifests from a
well-resolved IR spectrum, which was analyzed in terms of
individual vibrations on the basis of quasi-harmonic ab
initio phonon calculations.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {422 - Spin-based and quantum information (POF2-422) / 424 -
Exploratory materials and phenomena (POF2-424) / 542 -
Neutrons (POF2-542) / 544 - In-house Research with PNI
(POF2-544) / 54G - JCNS (POF2-54G24)},
pid = {G:(DE-HGF)POF2-422 / G:(DE-HGF)POF2-424 /
G:(DE-HGF)POF2-542 / G:(DE-HGF)POF2-544 /
G:(DE-HGF)POF2-54G24},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000317259900042},
doi = {10.1021/cg400054k},
url = {https://juser.fz-juelich.de/record/201202},
}