Gast ::
| Hauptseite > Publikationsdatenbank > Structure and Dynamics of Oligonucleotides in the Gas Phase > print |
| Hauptseite > Publikationsdatenbank > Structure and Dynamics of Oligonucleotides in the Gas Phase > print |
| 001 | 201331 | ||
| 005 | 20240625095115.0 | ||
| 024 | 7 | _ | |a 10.1002/anie.201406910 |2 doi |
| 024 | 7 | _ | |a 0044-8249 |2 ISSN |
| 024 | 7 | _ | |a 0570-0833 |2 ISSN |
| 024 | 7 | _ | |a 1433-7851 |2 ISSN |
| 024 | 7 | _ | |a 1521-3773 |2 ISSN |
| 024 | 7 | _ | |a WOS:000347238800011 |2 WOS |
| 024 | 7 | _ | |a altmetric:2913666 |2 altmetric |
| 024 | 7 | _ | |a pmid:25417598 |2 pmid |
| 037 | _ | _ | |a FZJ-2015-03628 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |0 P:(DE-HGF)0 |a Arcella, Annalisa |b 0 |
| 245 | _ | _ | |a Structure and Dynamics of Oligonucleotides in the Gas Phase |
| 260 | _ | _ | |a Weinheim |b Wiley-VCH |c 2015 |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1435066168_32633 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a article |2 DRIVER |
| 520 | _ | _ | |a By combining ion-mobility mass spectrometry experiments with sub-millisecond classical and ab initio molecular dynamics we fully characterized, for the first time, the dynamic ensemble of a model nucleic acid in the gas phase under electrospray ionization conditions. The studied oligonucleotide unfolds upon vaporization, loses memory of the solution structure, and explores true gas-phase conformational space. Contrary to our original expectations, the oligonucleotide shows very rich dynamics in three different timescales (multi-picosecond, nanosecond, and sub-millisecond). The shorter timescale dynamics has a quantum mechanical nature and leads to changes in the covalent structure, whereas theother two are of classical origin. Overall, this study suggests that a re-evaluation on our view of the physics of nucleic acids upon vaporization is needed. |
| 536 | _ | _ | |0 G:(DE-HGF)POF3-574 |a 574 - Theory, modelling and simulation (POF3-574) |c POF3-574 |f POF III |x 0 |
| 588 | _ | _ | |a Dataset connected to CrossRef, juser.fz-juelich.de |
| 700 | 1 | _ | |0 P:(DE-Juel1)146008 |a Dreyer, Jens |b 1 |u fzj |
| 700 | 1 | _ | |0 P:(DE-Juel1)146009 |a Ippoliti, Emiliano |b 2 |u fzj |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Ivani, Ivan |b 3 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Portella, Guillem |b 4 |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Gabelica, Valérie |b 5 |
| 700 | 1 | _ | |0 P:(DE-Juel1)145614 |a Carloni, Paolo |b 6 |u fzj |
| 700 | 1 | _ | |0 P:(DE-HGF)0 |a Orozco, Modesto |b 7 |e Corresponding Author |
| 773 | _ | _ | |0 PERI:(DE-600)2011836-3 |a 10.1002/anie.201406910 |g p. n/a - n/a |n 2 |p 467–471 |t Angewandte Chemie / International edition |v 54 |x 1433-7851 |y 2015 |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.pdf |y Restricted |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.gif?subformat=icon |x icon |y Restricted |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.jpg?subformat=icon-1440 |x icon-1440 |y Restricted |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.jpg?subformat=icon-180 |x icon-180 |y Restricted |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.jpg?subformat=icon-640 |x icon-640 |y Restricted |
| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/201331/files/467_ftp.pdf?subformat=pdfa |x pdfa |y Restricted |
| 909 | C | O | |o oai:juser.fz-juelich.de:201331 |p VDB |
| 910 | 1 | _ | |0 I:(DE-588b)5008462-8 |6 P:(DE-Juel1)146008 |a Forschungszentrum Jülich GmbH |b 1 |k FZJ |
| 910 | 1 | _ | |0 I:(DE-588b)5008462-8 |6 P:(DE-Juel1)146009 |a Forschungszentrum Jülich GmbH |b 2 |k FZJ |
| 910 | 1 | _ | |0 I:(DE-588b)5008462-8 |6 P:(DE-Juel1)145614 |a Forschungszentrum Jülich GmbH |b 6 |k FZJ |
| 913 | 0 | _ | |0 G:(DE-HGF)POF2-899 |1 G:(DE-HGF)POF2-890 |2 G:(DE-HGF)POF2-800 |a DE-HGF |b Programmungebundene Forschung |l ohne Programm |v ohne Topic |x 0 |
| 913 | 1 | _ | |0 G:(DE-HGF)POF3-574 |1 G:(DE-HGF)POF3-570 |2 G:(DE-HGF)POF3-500 |a DE-HGF |b Key Technologies |l Decoding the Human Brain |v Theory, modelling and simulation |x 0 |4 G:(DE-HGF)POF |3 G:(DE-HGF)POF3 |
| 914 | 1 | _ | |y 2015 |
| 915 | _ | _ | |0 StatID:(DE-HGF)0100 |2 StatID |a JCR |
| 915 | _ | _ | |0 StatID:(DE-HGF)0110 |2 StatID |a WoS |b Science Citation Index |
| 915 | _ | _ | |0 StatID:(DE-HGF)0111 |2 StatID |a WoS |b Science Citation Index Expanded |
| 915 | _ | _ | |0 StatID:(DE-HGF)0150 |2 StatID |a DBCoverage |b Web of Science Core Collection |
| 915 | _ | _ | |0 StatID:(DE-HGF)0199 |2 StatID |a DBCoverage |b Thomson Reuters Master Journal List |
| 915 | _ | _ | |0 StatID:(DE-HGF)0200 |2 StatID |a DBCoverage |b SCOPUS |
| 915 | _ | _ | |0 StatID:(DE-HGF)0300 |2 StatID |a DBCoverage |b Medline |
| 915 | _ | _ | |0 StatID:(DE-HGF)0310 |2 StatID |a DBCoverage |b NCBI Molecular Biology Database |
| 915 | _ | _ | |0 StatID:(DE-HGF)1030 |2 StatID |a DBCoverage |b Current Contents - Life Sciences |
| 915 | _ | _ | |0 StatID:(DE-HGF)1150 |2 StatID |a DBCoverage |b Current Contents - Physical, Chemical and Earth Sciences |
| 915 | _ | _ | |0 StatID:(DE-HGF)9910 |2 StatID |a IF >= 10 |
| 920 | _ | _ | |l yes |
| 920 | 1 | _ | |0 I:(DE-Juel1)INM-9-20140121 |k INM-9 |l Computational Biomedicine |x 0 |
| 920 | 1 | _ | |0 I:(DE-Juel1)IAS-5-20120330 |k IAS-5 |l Computational Biomedicine |x 1 |
| 920 | 1 | _ | |0 I:(DE-Juel1)GRS-20100316 |k GRS |l GRS |x 2 |
| 980 | _ | _ | |a journal |
| 980 | _ | _ | |a VDB |
| 980 | _ | _ | |a I:(DE-Juel1)INM-9-20140121 |
| 980 | _ | _ | |a I:(DE-Juel1)IAS-5-20120330 |
| 980 | _ | _ | |a I:(DE-Juel1)GRS-20100316 |
| 980 | _ | _ | |a UNRESTRICTED |
| 981 | _ | _ | |a I:(DE-Juel1)IAS-5-20120330 |
| 981 | _ | _ | |a I:(DE-Juel1)GRS-20100316 |
| Library | Collection | CLSMajor | CLSMinor | Language | Author |
|---|