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@ARTICLE{Kakudate:201499,
author = {Kakudate, Toshiyuki and Tsukamoto, Shigeru and Kubo, Osamu
and Nakaya, Masato and Nakayama, Tomonobu},
title = {{O}ctithiophene on {C}u(111) and {A}u(111): {F}ormation and
{E}lectronic {S}tructure of {M}olecular {C}hains and
{F}ilms},
journal = {Journal of nanoscience and nanotechnology},
volume = {12},
number = {5},
issn = {1533-4899},
address = {Stevenson Ranch, Calif.},
publisher = {American Scientific Publ.},
reportid = {FZJ-2015-03794},
pages = {4007 - 4011},
year = {2012},
abstract = {Adsorption and electronic structure of octithiophene (8T)
molecules on Cu(111) and Au(111) surfaces are investigated
using scanning tunneling microscopy (STM) and spectroscopy
(STS) at room temperature. We find a large difference in
adsorption behavior of 8T molecules on the two surfaces. At
the initial stage of adsorption, 8T molecules are stabilized
in the form of molecular chain on a terrace of Cu(111),
whereas neither such chain structure nor isolated 8T
molecules have been observed on a terrace of Au(111). By
increasing the amount of adsorbed molecules, a disordered
monolayer film is formed on Cu(111) while a well-ordered
monolayer film is formed on Au(111). From the spectroscopic
investigations using bias-dependent STM images and STS
spectra and by comparing the data with theoretical
calculations, it is found that the electronic property of 8T
molecules in the molecular chain on Cu(111) is different
from that of a free-standing 8T molecule while that in the
monolayer film on Au(111) keeps original character of the
free-standing 8T molecule. The present study shows that
adsorption of 8T molecules on Cu(111) results in a formation
of adsorption-induced states near the Fermi level.},
cin = {IAS-1 / PGI-1},
ddc = {540},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106},
pnm = {422 - Spin-based and quantum information (POF2-422)},
pid = {G:(DE-HGF)POF2-422},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000305851000043},
doi = {10.1166/jnn.2012.5860},
url = {https://juser.fz-juelich.de/record/201499},
}