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@ARTICLE{Schmale:201539,
author = {Schmale, K. and Barthel, J. and Bernemann, M. and
Grünebaum, M. and Koops, S. and Schmidt, Marita and Mayer,
J. and Wiemhöfer, H. -D.},
title = {{AFM} investigations on the influence of {C}$_{{O}2}$
exposure on
{B}a$_{0.5}${S}r$_{0.5}${C}o$_{0.8}${F}e$_{0.2}${O}$_{3–δ}$},
journal = {Journal of solid state electrochemistry},
volume = {17},
number = {11},
issn = {1433-0768},
address = {Berlin},
publisher = {Springer},
reportid = {FZJ-2015-03833},
pages = {2897 - 2907},
year = {2013},
abstract = {In this work, fresh and CO2-exposed specimens of
Ba0.5Sr0.5Co0.8Fe0.2O3–δ (BSCF) are examined by atomic
force microscopy (AFM) using amplitude-modulated Kelvin
probe force microscopy (KPFM) and also electrostatic force
microscopy (EFM) to characterize the early stages of the
formation of reaction products due to reaction with gaseous
CO2. A comparison is made with results from electron
microscopy on the same samples. BSCF specimens exposed for
24 and 240 h to an atmosphere of 99.9 $\%$ CO2 at 900 °C,
respectively, were analyzed and compared with non-exposed
specimens. The observation of interconnected carbonate
islands on BSCF forming a continuous carbonate layer after
some exposure to CO2 indicates a Stranski–Krastanov or
Volmer–Weber growth mechanism of the carbonate layer. Our
results demonstrate that the measurement of surface
potential variations by means of KPFM and EFM constitutes a
very sensitive technique to detect the formation of reaction
layers on gas permeation membranes such as BSCF. In contrast
to electron microscopy techniques, scanning probe techniques
permit the investigation of the topography and of
electrochemical characteristics of the sample surface as
received and without further preparation.},
cin = {PGI-5},
ddc = {540},
cid = {I:(DE-Juel1)PGI-5-20110106},
pnm = {42G - Peter Grünberg-Centre (PG-C) (POF2-42G41)},
pid = {G:(DE-HGF)POF2-42G41},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000325615000019},
doi = {10.1007/s10008-013-2159-3},
url = {https://juser.fz-juelich.de/record/201539},
}