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@ARTICLE{Sivebaek:201805,
author = {Sivebaek, I. M. and Samoilov, V. N. and Persson, Bo},
title = {{E}ffective {V}iscosity of {C}onfined {H}ydrocarbons},
journal = {Physical review letters},
volume = {108},
number = {3},
issn = {1079-7114},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2015-04099},
pages = {036102},
year = {2012},
abstract = {We present molecular dynamics friction calculations for
confined hydrocarbon films with molecular lengths from 20 to
1400 carbon atoms. We find that the logarithm of the
effective viscosity ηeff for nanometer-thin films depends
linearly on the logarithm of the shear rate:
logηeff=C−nlogγ˙, where n varies from 1
(solidlike friction) at very low temperatures to 0
(Newtonian liquid) at very high temperatures, following an
inverse sigmoidal curve. Only the shortest chain molecules
melt, whereas the longer ones only show a softening in the
studied temperature interval 0<T<900 K. The results are
important for the frictional properties of very thin
(nanometer) films and to estimate their thermal durability.},
cin = {IAS-1 / PGI-1},
ddc = {550},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106},
pnm = {424 - Exploratory materials and phenomena (POF2-424)},
pid = {G:(DE-HGF)POF2-424},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000299329100019},
doi = {10.1103/PhysRevLett.108.036102},
url = {https://juser.fz-juelich.de/record/201805},
}