000201869 001__ 201869
000201869 005__ 20210129215934.0
000201869 0247_ $$2doi$$a10.1038/ncomms6441
000201869 0247_ $$2WOS$$aWOS:000345908900001
000201869 0247_ $$2altmetric$$aaltmetric:2943563
000201869 0247_ $$2pmid$$apmid:25399688
000201869 0247_ $$2Handle$$a2128/24461
000201869 037__ $$aFZJ-2015-04163
000201869 082__ $$a500
000201869 1001_ $$0P:(DE-HGF)0$$aNemšák, Slavomír$$b0$$eCorresponding Author
000201869 245__ $$aConcentration and chemical-state profiles at heterogeneous interfaces with sub-nm accuracy from standing-wave ambient-pressure photoemission
000201869 260__ $$aLondon$$bNature Publishing Group$$c2014
000201869 3367_ $$2DRIVER$$aarticle
000201869 3367_ $$2DataCite$$aOutput Types/Journal article
000201869 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1435643663_1776
000201869 3367_ $$2BibTeX$$aARTICLE
000201869 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000201869 3367_ $$00$$2EndNote$$aJournal Article
000201869 520__ $$aHeterogeneous processes at solid/gas, liquid/gas and solid/liquid interfaces are ubiquitous in modern devices and technologies but often difficult to study quantitatively. Full characterization requires measuring the depth profiles of chemical composition and state with enhanced sensitivity to narrow interfacial regions of a few to several nm in extent over those originating from the bulk phases on either side of the interface. We show for a model system of ​NaOH and ​CsOH in an ~1-nm thick hydrated layer on α-Fe2O3 (haematite) that combining ambient-pressure X-ray photoelectron spectroscopy and standing-wave photoemission spectroscopy provides the spatial arrangement of the bulk and interface chemical species, as well as local potential energy variations, along the direction perpendicular to the interface with sub-nm accuracy. Standing-wave ambient-pressure photoemission spectroscopy is thus a very promising technique for measuring such important interfaces, with relevance to energy research, heterogeneous catalysis, electrochemistry, and atmospheric and environmental science.
000201869 536__ $$0G:(DE-HGF)POF2-422$$a422 - Spin-based and quantum information (POF2-422)$$cPOF2-422$$fPOF II$$x0
000201869 588__ $$aDataset connected to CrossRef, juser.fz-juelich.de
000201869 7001_ $$0P:(DE-HGF)0$$aShavorskiy, Andrey$$b1
000201869 7001_ $$0P:(DE-HGF)0$$aKarslioglu, Osman$$b2
000201869 7001_ $$0P:(DE-HGF)0$$aZegkinoglou, Ioannis$$b3
000201869 7001_ $$0P:(DE-HGF)0$$aRattanachata, Arunothai$$b4
000201869 7001_ $$0P:(DE-HGF)0$$aConlon, Catherine S.$$b5
000201869 7001_ $$0P:(DE-HGF)0$$aKeqi, Armela$$b6
000201869 7001_ $$0P:(DE-HGF)0$$aGreene, Peter K.$$b7
000201869 7001_ $$0P:(DE-HGF)0$$aBurks, Edward C.$$b8
000201869 7001_ $$0P:(DE-HGF)0$$aSalmassi, Farhad$$b9
000201869 7001_ $$0P:(DE-HGF)0$$aGullikson, Eric M.$$b10
000201869 7001_ $$0P:(DE-HGF)0$$aYang, See-Hun$$b11
000201869 7001_ $$0P:(DE-HGF)0$$aLiu, Kai$$b12
000201869 7001_ $$0P:(DE-HGF)0$$aBluhm, Hendrik$$b13$$eCorresponding Author
000201869 7001_ $$0P:(DE-HGF)0$$aFadley, Charles S.$$b14$$eCorresponding Author
000201869 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/ncomms6441$$gVol. 5, p. 5441 -$$p5441 -$$tNature Communications$$v5$$x2041-1723$$y2014
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.pdf$$yOpenAccess
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.gif?subformat=icon$$xicon$$yOpenAccess
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000201869 8564_ $$uhttps://juser.fz-juelich.de/record/201869/files/ncomms6441.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000201869 909CO $$ooai:juser.fz-juelich.de:201869$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000201869 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-HGF)0$$aForschungszentrum Jülich GmbH$$b0$$kFZJ
000201869 9132_ $$0G:(DE-HGF)POF3-522$$1G:(DE-HGF)POF3-520$$2G:(DE-HGF)POF3-500$$aDE-HGF$$bKey Technologies$$lFuture Information Technology - Fundamentals, Novel Concepts and Energy Efficiency (FIT)$$vControlling Spin-Based Phenomena$$x0
000201869 9131_ $$0G:(DE-HGF)POF2-422$$1G:(DE-HGF)POF2-420$$2G:(DE-HGF)POF2-400$$3G:(DE-HGF)POF2$$4G:(DE-HGF)POF$$aDE-HGF$$bSchlüsseltechnologien$$lGrundlagen zukünftiger Informationstechnologien$$vSpin-based and quantum information$$x0
000201869 9141_ $$y2015
000201869 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000201869 915__ $$0StatID:(DE-HGF)1030$$2StatID$$aDBCoverage$$bCurrent Contents - Life Sciences
000201869 915__ $$0StatID:(DE-HGF)1040$$2StatID$$aDBCoverage$$bZoological Record
000201869 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR
000201869 915__ $$0StatID:(DE-HGF)9910$$2StatID$$aIF >= 10
000201869 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000201869 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000201869 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000201869 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000201869 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000201869 915__ $$0StatID:(DE-HGF)1060$$2StatID$$aDBCoverage$$bCurrent Contents - Agriculture, Biology and Environmental Sciences
000201869 915__ $$0StatID:(DE-HGF)0310$$2StatID$$aDBCoverage$$bNCBI Molecular Biology Database
000201869 915__ $$0StatID:(DE-HGF)1050$$2StatID$$aDBCoverage$$bBIOSIS Previews
000201869 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000201869 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bThomson Reuters Master Journal List
000201869 9201_ $$0I:(DE-Juel1)PGI-6-20110106$$kPGI-6$$lElektronische Eigenschaften$$x0
000201869 980__ $$ajournal
000201869 980__ $$aVDB
000201869 980__ $$aUNRESTRICTED
000201869 980__ $$aI:(DE-Juel1)PGI-6-20110106
000201869 9801_ $$aFullTexts