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000020193 084__ $$2WoS$$aChemistry, Physical
000020193 084__ $$2WoS$$aPhysics, Atomic, Molecular & Chemical
000020193 1001_ $$0P:(DE-HGF)0$$aHaiser, K.$$b0
000020193 245__ $$aNitro-Phenylalanine: A Novel Sensor for Heat Transfer in Peptides
000020193 260__ $$aWashington, DC$$bSoc.$$c2011
000020193 300__ $$a2169 - 2175
000020193 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article
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000020193 440_0 $$03693$$aJournal of Physical Chemistry A$$v115$$x1089-5639$$y11
000020193 500__ $$aThis work was supported by the Deutsche Forschungsgemeinschaft through the DFG-Cluster of Excellence Munich-Centre for Advanced Photonics and SFB 749 (A5).
000020193 520__ $$aFemtosecond IR-pump-IR-probe experiments with independently tunable pulses are used to monitor the ultrafast response of selected IR absorption bands to vibrational excitation of other modes of Fmoc-nitrophenylalanine. The absorptions of both NO(2)-bands change rapidly within <2 ps upon excitation of other vibrational modes. The results point to considerable coupling between the monitored NO(2) modes and the initially excited modes or low-frequency modes. The latter are populated by a rapid energy redistribution process. The strong IR absorption of the NO(2) stretching bands and the intense coupling to other modes makes the nitro group of nitrophenylalanine a sensitive monitor for vibrational energy arriving at this amino acid.
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000020193 588__ $$aDataset connected to Web of Science, Pubmed
000020193 650_2 $$2MeSH$$aEnergy Transfer
000020193 650_2 $$2MeSH$$aHot Temperature
000020193 650_2 $$2MeSH$$aPeptides: chemistry
000020193 650_2 $$2MeSH$$aPhenylalanine: analogs & derivatives
000020193 650_2 $$2MeSH$$aSpectrophotometry, Infrared: instrumentation
000020193 650_2 $$2MeSH$$aVibration
000020193 650_7 $$00$$2NLM Chemicals$$aPeptides
000020193 650_7 $$01991-83-9$$2NLM Chemicals$$a4-nitrophenylalanine
000020193 650_7 $$063-91-2$$2NLM Chemicals$$aPhenylalanine
000020193 650_7 $$2WoSType$$aJ
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000020193 7001_ $$0P:(DE-HGF)0$$aKoller, F.O.$$b1
000020193 7001_ $$0P:(DE-HGF)0$$aHuber, M.$$b2
000020193 7001_ $$0P:(DE-HGF)0$$aRegner, N.$$b3
000020193 7001_ $$0P:(DE-Juel1)138266$$aSchrader, T.E.$$b4$$uFZJ
000020193 7001_ $$0P:(DE-HGF)0$$aSchreier, W.J.$$b5
000020193 7001_ $$0P:(DE-HGF)0$$aZinth, W.$$b6
000020193 773__ $$0PERI:(DE-600)2006031-2$$a10.1021/jp110597a$$gVol. 115, p. 2169 - 2175$$p2169 - 2175$$q115<2169 - 2175$$tThe @journal of physical chemistry <Washington, DC> / A$$v115$$x1089-5639$$y2011
000020193 8567_ $$uhttp://dx.doi.org/10.1021/jp110597a
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