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@ARTICLE{Xiao:202214,
author = {Xiao, Bin and Klinkenberg, Martina and Bosbach, Dirk and
Suleimanov, Evgeny V. and Alekseev, Evgeny},
title = {{E}ffects of {T}e({IV}) {O}xo-{A}nion {I}ncorporation into
{T}horium {M}olybdates and {T}ungstates},
journal = {Inorganic chemistry},
volume = {54},
number = {12},
issn = {1520-510X},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {FZJ-2015-04503},
pages = {5981 - 5990},
year = {2015},
abstract = {The exploration of phase formation in the Th−Mo/W−Te
systems has resulted in four mixed oxo-anion compounds from
high-temperature solid-state reactions:ThWTe2O9,
Th(WO4)(TeO3), ThMoTe2O9, and Th2(MoO4)-(TeO3)3. All four
compounds contain edge-sharing thorium polyhedra linked by
MoO4/WO6 and different tellurium oxogroups to form
three-dimensional frameworks. In ThWTe2O9, each helical Th
based chain is connected by four tungstotellurite clusters
resulting in a building fragment which has a crosssection of
four-leafed clovers. The structure of Th(WO4)(TeO3) exhibits
a multilayer-sandwich framework composed of thorium
tellurite layers with tungsten chains in between. In the
case of the molybdate family, ThMoTe2O9 and Th2(MoO4)(TeO3)3
are built from puckered Th−Te sheets which are further
interconnected by MoO4 tetrahedral linkers. The DSC-TG
technique was performed to gain insight into the thermal
behavior of the synthesized compounds. Raman spectra of
as-prepared phases were obtained and analyzed for signature
peaks.},
cin = {IEK-6},
ddc = {540},
cid = {I:(DE-Juel1)IEK-6-20101013},
pnm = {161 - Nuclear Waste Management (POF3-161) / Helmholtz Young
Investigators Group: Energy (HGF-YIG-Energy) / HITEC -
Helmholtz Interdisciplinary Doctoral Training in Energy and
Climate Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF3-161 / G:(DE-HGF)HGF-YIG-Energy /
G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000356467100039},
pubmed = {pmid:26020835},
doi = {10.1021/acs.inorgchem.5b00789},
url = {https://juser.fz-juelich.de/record/202214},
}