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@ARTICLE{Doanay:202817,
author = {Doğanay, H. and Krug, Ingo and Schubert, J. and Cramm, S.
and Gottlob, Daniel and Nickel, Florian and Schneider, C.
M.},
title = {{T}uning the orbital ordering in {L}a 0.7 {S}r 0.3 {M}n{O}
3 thin films in all-oxide hybrids},
journal = {epl},
volume = {109},
number = {6},
issn = {1286-4854},
address = {Les Ulis},
publisher = {EDP Sciences},
reportid = {FZJ-2015-04978},
pages = {67007 -},
year = {2015},
abstract = {This work presents a systematic characterization including
x-ray diffractometry,SQUID magnetometry and x-ray absorption
spectroscopy on all-oxide
ferromagnetic/ferroelectricheterosystem
BaTiO3/La0.7Sr0.3MnO3/SrTiO3(001) fabricated by pulsed-laser
deposition. Thekey aspect of this study is to provide
accurate information about differences in electronic
andstructural properties in LSMO thin films as a function of
the oxygen pressure during BTO growth.X-ray absorption
spectroscopy experiments at the Mn L3,2 edge have revealed
the conservation ofMn3+/Mn4+ mixed valency configuration of
the LSMO films near the interface while tuning theoxygen
pressure of overlayer BTO growth. The existing Mn3+ ions
favor an in-plane eg orbitalordering, reducing the in-plane
strain and promoting room temperature ferromagntism in
theLSMO film. Furthermore, diffraction experiments showed
that the out-of plane lattice parameterof BTO reduces with
increasing oxygen pressure consistent with the x-ray linear
dichrosim at Tiedge showing less tetragonal symmetry,
although the chemical environment of the Ti ions was
notchanged notably. We demonstrated a way to control
magnetic properties and orbital ordering inLSMO thin films
while optimizing the ferroelectric properties of BTO
overlayer films, which arepromising results in terms of
magnetoelectric applications using functional
heterosystems.},
cin = {PGI-6 / PGI-9 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)PGI-6-20110106 / I:(DE-Juel1)PGI-9-20110106 /
$I:(DE-82)080009_20140620$},
pnm = {521 - Controlling Electron Charge-Based Phenomena
(POF3-521)},
pid = {G:(DE-HGF)POF3-521},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000355579000018},
doi = {10.1209/0295-5075/109/67007},
url = {https://juser.fz-juelich.de/record/202817},
}