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000203324 1001_ $$0P:(DE-HGF)0$$aZhuang, Hao$$b0
000203324 245__ $$aDiamond Network: Template-Free Fabrication and Properties
000203324 260__ $$aWashington, DC$$bSoc.$$c2015
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000203324 520__ $$aA porous diamond network with three-dimensionally interconnected pores is of technical importance but difficult to be produced. In this contribution, we demonstrate a simple, controllable, and “template-free” approach to fabricate diamond networks. It combines the deposition of diamond/β-SiC nanocomposite film with a wet-chemical selective etching of the β-SiC phase. The porosity of these networks was tuned from 15 to 68%, determined by the ratio of the β-SiC phase in the composite films. The electrochemical working potential and the reactivity of redox probes on the diamond networks are similar to those of a flat nanocrystalline diamond film, while their surface areas are hundreds of times larger than that of a flat diamond film (e.g., 490-fold enhancement for a 3 μm thick diamond network). The marriage of the unprecedented physical/chemical features of diamond with inherent advantages of the porous structure makes the diamond network a potential candidate for various applications such as water treatment, energy conversion (batteries or fuel cells), and storage (capacitors), as well as electrochemical and biochemical sensing.
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000203324 7001_ $$0P:(DE-HGF)0$$aYang, Nianjun$$b1
000203324 7001_ $$0P:(DE-HGF)0$$aFu, Haiyuan$$b2
000203324 7001_ $$0P:(DE-Juel1)140353$$aZhang, Lei$$b3
000203324 7001_ $$0P:(DE-HGF)0$$aWang, Chun$$b4
000203324 7001_ $$0P:(DE-HGF)0$$aHuang, Nan$$b5
000203324 7001_ $$0P:(DE-HGF)0$$aJiang, Xin$$b6$$eCorresponding author
000203324 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/am508851r$$gVol. 7, no. 9, p. 5384 - 5390$$n9$$p5384 - 5390$$tACS applied materials & interfaces$$v7$$x1944-8252$$y2015
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