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000203325 1001_ $$0P:(DE-HGF)0$$aMa, Yao$$b0
000203325 245__ $$aShape-Controlled Growth of Carbon Nanostructures: Yield and Mechanism
000203325 260__ $$aWeinheim$$bWiley-VCH$$c2015
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000203325 520__ $$aCarbon nanostructures with precisely controlled shapes are difficult materials to synthesize. A facet-selective-catalytic process was thus proposed to synthesize polymer-linked carbon nanostructures with different shapes, covering straight carbon nanofiber, carbon nano Y-junction, carbon nano-hexapus, and carbon nano-octopus. A thermal chemical vapor deposition process was applied to grow these multi-branched carbon nanostructures at temperatures lower than 350 °C. Cu nanoparticles were utilized as the catalyst and acetylene as the reaction gas. The growth of those multi-branched nanostructures was realized through the selective growth of polymer-like sheets on certain indexed facets of Cu catalyst. The vapor–facet–solid (VFS) mechanism, a new growth mode, has been proposed to interpret such a growth in the steps of formation, diffusion, and coupling of carbon-containing oligomers, as well as their final precipitation to form nanostructures on the selective Cu facets.
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000203325 7001_ $$0P:(DE-Juel1)151305$$aSun, Xiao$$b1
000203325 7001_ $$0P:(DE-HGF)0$$aYang, Nianjun$$b2$$eCorresponding author
000203325 7001_ $$0P:(DE-HGF)0$$aXia, Junhai$$b3
000203325 7001_ $$0P:(DE-Juel1)140353$$aZhang, Lei$$b4
000203325 7001_ $$0P:(DE-HGF)0$$aJiang, Xin$$b5
000203325 773__ $$0PERI:(DE-600)1478547-x$$a10.1002/chem.201500440$$gVol. 21, no. 35, p. 12370 - 12375$$n35$$p12370 - 12375$$tChemistry - a European journal$$v21$$x0947-6539$$y2015
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