000203426 001__ 203426 000203426 005__ 20240610120559.0 000203426 0247_ $$2doi$$a10.1016/j.jallcom.2015.08.135 000203426 0247_ $$2ISSN$$a0925-8388 000203426 0247_ $$2ISSN$$a1873-4669 000203426 0247_ $$2WOS$$aWOS:000361830700076 000203426 037__ $$aFZJ-2015-05367 000203426 041__ $$aEnglish 000203426 082__ $$a670 000203426 1001_ $$0P:(DE-Juel1)144017$$aSchäfer, Anna$$b0 000203426 245__ $$aPolymorphous GdScO$_{3}$ as high permittivity dielectric 000203426 260__ $$aLausanne$$bElsevier$$c2015 000203426 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1446648314_12656 000203426 3367_ $$2DataCite$$aOutput Types/Journal article 000203426 3367_ $$00$$2EndNote$$aJournal Article 000203426 3367_ $$2BibTeX$$aARTICLE 000203426 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000203426 3367_ $$2DRIVER$$aarticle 000203426 520__ $$aFour different polymorphs of GdScO3 are assessed theoretically and experimentally with respectto their suitability as a dielectric. The calculations carried out by density functional theory reveallattice constants, band gaps and the energies of formation of three crystal phases. Experimentallyall three crystal phases and the amorphous phase can be realized as thin films by pulsed laserdeposition using various growth templates. Their respective crystal structures are confirmed byx-ray diffraction and transmission electron microscopy reflecting the calculated lattice constants.X-ray photoelectron spectroscopy unveils the band gaps of the different polymorphs of GdScO3which are above 5 eV for all films demonstrating good insulating properties. From capacitancevoltage measurements, high permittivities of up to 27 for hexagonal GdScO3 are deduced. 000203426 536__ $$0G:(DE-HGF)POF3-142$$a142 - Controlling Spin-Based Phenomena (POF3-142)$$cPOF3-142$$fPOF III$$x0 000203426 536__ $$0G:(DE-HGF)POF3-521$$a521 - Controlling Electron Charge-Based Phenomena (POF3-521)$$cPOF3-521$$fPOF III$$x1 000203426 588__ $$aDataset connected to CrossRef 000203426 7001_ $$0P:(DE-Juel1)130906$$aRahmanizadeh, K.$$b1 000203426 7001_ $$0P:(DE-Juel1)130545$$aBihlmayer, G.$$b2 000203426 7001_ $$0P:(DE-Juel1)130811$$aLuysberg, M.$$b3 000203426 7001_ $$0P:(DE-Juel1)161187$$aWendt, F.$$b4 000203426 7001_ $$0P:(DE-Juel1)133839$$aBesmehn, A.$$b5 000203426 7001_ $$0P:(DE-Juel1)125583$$aFox, A.$$b6 000203426 7001_ $$0P:(DE-Juel1)139578$$aSchnee, M.$$b7 000203426 7001_ $$0P:(DE-HGF)0$$aNiu, G.$$b8 000203426 7001_ $$0P:(DE-HGF)0$$aSchroeder, T.$$b9 000203426 7001_ $$0P:(DE-Juel1)128609$$aMantl, S.$$b10 000203426 7001_ $$0P:(DE-Juel1)125593$$aHardtdegen, H.$$b11 000203426 7001_ $$0P:(DE-Juel1)128613$$aMikulics, M.$$b12 000203426 7001_ $$0P:(DE-Juel1)128631$$aSchubert, J.$$b13$$eCorresponding author 000203426 773__ $$0PERI:(DE-600)2012675-X$$a10.1016/j.jallcom.2015.08.135$$gp. 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