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@ARTICLE{Valldor:20465,
author = {Valldor, M. and Hermann, R. and Wuttke, J. and Zamponi, M.
and Schweika, W.},
title = {{S}pin correlation in the extended kagome system
{Y}ba{C}o3{F}e{O}7},
journal = {Physical review / B},
volume = {84},
number = {22},
issn = {1098-0121},
address = {College Park, Md.},
publisher = {APS},
reportid = {PreJuSER-20465},
pages = {224426},
year = {2011},
note = {We are grateful for comments from Daniel Khomskii and Gary
J. Long. Moulay Sougrati is acknowledged for assisting in
the collection of the Mossbauer spectral data. We would like
to thank Anne Mochel for help in measuring magnetic
susceptibility of the isotope-enriched sample. This work was
supported by DFG through the project SFB 608, by the FNRS
through Grants No. 9.456595 and 1.5.064.5, and by the
Helmholtz Association of German Research Centers through
Grant No. NG-407. Part of this research at the instrument
BASIS Oak Ridge National Laboratories Spallation Neutron
Source was sponsored by the Scientific User Facilities
Division, Office of Basic Energy Sciences, US Department of
Energy.},
abstract = {The transition metal-based oxide YBaCo3FeO7 is structurally
related to the mineral Swedenborgite SbNaBe4O7, a polar
noncentrosymmetric crystal system. The magnetic Co3Fe
sublattice consists of a tetrahedral network containing
kagome-like layers with trigonal interlayer sites. This
geometry causes frustration effects for magnetic ordering,
which were investigated by magnetization measurements,
Mossbauer spectroscopy, polarized neutron diffraction, and
neutron spectroscopy. Magnetization measurement and neutron
diffraction do not show long range ordering even at low
temperature (1 K), although a strong antiferromagnetic
coupling (similar to 2000 K) is deduced from the magnetic
susceptibility. Below 590 K we observe two features, a
spontaneous weak anisotropic magnetization hysteresis along
the polar crystallographic axis and a hyperfine field on the
Fe kagome sites, whereas the Fe spins on the interlayer
sites remain idle. Below similar to 50 K the onset of a
hyperfine field shows the development of moments static on
the Mossbauer time scale also for the Fe interlayer sites.
Simultaneously, an increase of spin correlations is found by
polarized neutron diffraction. The relaxation part of the
dynamic response has been further investigated by
high-resolution neutron spectroscopy, which reveals that the
spin correlations start to freeze below similar to 50 K.
Monte Carlo simulations show that the neutron scattering
results at lower temperatures are compatible with a recent
proposal that the particular geometric frustration in the
Swedenborgite structure promotes quasi-one-dimensional
partial order.},
keywords = {J (WoSType)},
cin = {PGI-4 / JCNS-2 / JARA-FIT / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {530},
cid = {I:(DE-Juel1)PGI-4-20110106 / I:(DE-Juel1)JCNS-2-20110106 /
$I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {Grundlagen für zukünftige Informationstechnologien},
pid = {G:(DE-Juel1)FUEK412},
experiment = {EXP:(DE-MLZ)DNS-20140101 / EXP:(DE-MLZ)SPHERES-20140101},
shelfmark = {Physics, Condensed Matter},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000298556000008},
doi = {10.1103/PhysRevB.84.224426},
url = {https://juser.fz-juelich.de/record/20465},
}