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@ARTICLE{Yang:20544,
      author       = {Yang, M. and Ripoll, M.},
      title        = {{D}riving forces and polymer hydrodynamics in the {S}oret
                      effect},
      journal      = {Journal of physics / Condensed matter},
      volume       = {24},
      issn         = {0953-8984},
      address      = {Bristol},
      publisher    = {IOP Publ.},
      reportid     = {PreJuSER-20544},
      pages        = {195101},
      year         = {2012},
      note         = {Record converted from VDB: 12.11.2012},
      abstract     = {A temperature gradient induces different driving forces on
                      the components of a mixture which translates into their
                      segregation. We show that these driving forces constitute
                      the physical picture behind the thermodiffusion effect, and
                      provide an alternative expression of the Soret coefficient
                      which can be applied to both colloidal suspensions and
                      molecular mixtures. To verify the validity of the formalism,
                      we quantify the related forces in an Eulerian reference
                      frame by non-equilibrium molecular simulations. Furthermore,
                      we present an analytical argument to show that the
                      hydrodynamic interactions need to be accounted for to obtain
                      the proper scaling of the thermophoretic force. This result
                      combined with the presented expression satisfactorily
                      explains the experimentally known size dependence of the
                      thermodiffusion coefficient in dilute polymer solutions.},
      keywords     = {Diffusion / Hydrodynamics / Models, Theoretical / Polymers:
                      chemistry / Reproducibility of Results / Solutions /
                      Temperature / Polymers (NLM Chemicals) / Solutions (NLM
                      Chemicals) / J (WoSType)},
      cin          = {ICS-2},
      ddc          = {530},
      cid          = {I:(DE-Juel1)ICS-2-20110106},
      pnm          = {BioSoft: Makromolekulare Systeme und biologische
                      Informationsverarbeitung},
      pid          = {G:(DE-Juel1)FUEK505},
      shelfmark    = {Physics, Condensed Matter},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:22466869},
      UT           = {WOS:000303501000003},
      doi          = {10.1088/0953-8984/24/19/195101},
      url          = {https://juser.fz-juelich.de/record/20544},
}